Quantum-Phase Electronics Center (QPEC) and Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan.
Quantum-Phase Electronics Center (QPEC) and Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan. Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG, Groningen, Netherlands. RIKEN Center for Emergent Matter Science (CEMS), Wako 351-0198, Japan.
Science. 2014 May 16;344(6185):725-8. doi: 10.1126/science.1251329. Epub 2014 Apr 17.
Tungsten diselenide (WSe2) and related transition metal dichalcogenides exhibit interesting optoelectronic properties owing to their peculiar band structures originating from the valley degree of freedom. Although the optical generation and detection of valley polarization has been demonstrated, it has been difficult to realize active valley-dependent functions suitable for device applications. We report an electrically switchable, circularly polarized light source based on the material's valley degree of freedom. Our WSe2-based ambipolar transistors emit circularly polarized electroluminescence from p-i-n junctions electrostatically formed in transistor channels. This phenomenon can be explained qualitatively by the electron-hole overlap controlled by the in-plane electric field. Our device demonstrates a route to exploit the valley degree of freedom and the possibility to develop a valley-optoelectronics technology.
二硒化钨(WSe2)和相关的过渡金属二卤化物由于其独特的能带结构源于谷自由度而表现出有趣的光电特性。尽管已经证明了谷极化的光产生和检测,但很难实现适用于器件应用的有源谷相关功能。我们报告了一种基于材料谷自由度的电可切换圆偏振光源。我们基于 WSe2 的双极性晶体管从晶体管通道中静电形成的 p-i-n 结发射圆偏振电致发光。这种现象可以通过平面内电场控制的电子-空穴重叠来定性解释。我们的器件展示了一种利用谷自由度的途径,并有可能开发谷光电技术。