School of Engineering and Applied Sciences, Harvard University, 33 Oxford Street, Cambridge, Massachusetts 02138, USA.
Department of Physics, Columbia University, New York, New York 10027, USA.
Nat Nanotechnol. 2014 Aug;9(8):594-9. doi: 10.1038/nnano.2014.112. Epub 2014 Jun 22.
Individual electrons in graphene behave as massless quasiparticles. Unexpectedly, it is inferred from plasmonic investigations that electrons in graphene must exhibit a non-zero mass when collectively excited. The inertial acceleration of the electron collective mass is essential to explain the behaviour of plasmons in this material, and may be directly measured by accelerating it with a time-varying voltage and quantifying the phase delay of the resulting current. This voltage-current phase relation would manifest as a kinetic inductance, representing the reluctance of the collective mass to accelerate. However, at optical (infrared) frequencies, phase measurements of current are generally difficult, and, at microwave frequencies, the inertial phase delay has been buried under electron scattering. Therefore, to date, the collective mass in graphene has defied unequivocal measurement. Here, we directly and precisely measure the kinetic inductance, and therefore the collective mass, by combining device engineering that reduces electron scattering and sensitive microwave phase measurements. Specifically, the encapsulation of graphene between hexagonal boron nitride layers, one-dimensional edge contacts and a proximate top gate configured as microwave ground together enable the inertial phase delay to be resolved from the electron scattering. Beside its fundamental importance, the kinetic inductance is found to be orders of magnitude larger than the magnetic inductance, which may be utilized to miniaturize radiofrequency integrated circuits. Moreover, its bias dependency heralds a solid-state voltage-controlled inductor to complement the prevalent voltage-controlled capacitor.
在石墨烯中,单个电子表现为无质量的准粒子。出人意料的是,从等离子体研究推断,当电子集体激发时,它们必须表现出非零质量。电子集体质量的惯性加速度对于解释这种材料中的等离子体行为至关重要,并且可以通过用时变电压加速它并量化产生的电流的相位延迟来直接测量。这种电压-电流相位关系将表现为动力学电感,表示集体质量对加速的阻力。然而,在光学(红外)频率下,电流的相位测量通常很困难,而在微波频率下,惯性相位延迟已被电子散射所掩盖。因此,迄今为止,石墨烯中的集体质量一直难以进行明确的测量。在这里,我们通过结合减少电子散射的器件工程和灵敏的微波相位测量,直接和精确地测量了动力学电感,从而测量了集体质量。具体来说,将石墨烯夹在六方氮化硼层之间、一维边缘接触和邻近的顶部栅极配置为微波地,这使得可以从电子散射中分辨出惯性相位延迟。除了其基本重要性之外,动力学电感比磁电感大几个数量级,这可能用于缩小射频集成电路。此外,其偏置依赖性预示着一种固态电压控制电感器,可以补充流行的电压控制电容器。