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美国西南部气态氧化汞干沉降测量:德克萨斯州、俄克拉荷马州东部和四角地区之间的比较。

Gaseous oxidized mercury dry deposition measurements in the southwestern USA: a comparison between Texas, eastern Oklahoma, and the Four Corners area.

作者信息

Sather Mark E, Mukerjee Shaibal, Allen Kara L, Smith Luther, Mathew Johnson, Jackson Clarence, Callison Ryan, Scrapper Larry, Hathcoat April, Adam Jacque, Keese Danielle, Ketcher Philip, Brunette Robert, Karlstrom Jason, Van der Jagt Gerard

机构信息

Air Quality Analysis Section, US Environmental Protection Agency (EPA) Region 6, 1445 Ross Avenue, Dallas, TX 75202, USA.

National Exposure Research Laboratory, US EPA (E205-03), Research Triangle Park, NC 27711, USA.

出版信息

ScientificWorldJournal. 2014;2014:580723. doi: 10.1155/2014/580723. Epub 2014 Apr 6.

DOI:10.1155/2014/580723
PMID:24955412
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3997905/
Abstract

Gaseous oxidized mercury (GOM) dry deposition measurements using aerodynamic surrogate surface passive samplers were collected in central and eastern Texas and eastern Oklahoma, from September 2011 to September 2012. The purpose of this study was to provide an initial characterization of the magnitude and spatial extent of ambient GOM dry deposition in central and eastern Texas for a 12-month period which contained statistically average annual results for precipitation totals, temperature, and wind speed. The research objective was to investigate GOM dry deposition in areas of Texas impacted by emissions from coal-fired utility boilers and compare it with GOM dry deposition measurements previously observed in eastern Oklahoma and the Four Corners area. Annual GOM dry deposition rate estimates were relatively low in Texas, ranging from 0.1 to 0.3 ng/m(2)h at the four Texas monitoring sites, similar to the 0.2 ng/m(2)h annual GOM dry deposition rate estimate recorded at the eastern Oklahoma monitoring site. The Texas and eastern Oklahoma annual GOM dry deposition rate estimates were at least four times lower than the highest annual GOM dry deposition rate estimate previously measured in the more arid bordering western states of New Mexico and Colorado in the Four Corners area.

摘要

2011年9月至2012年9月期间,在得克萨斯州中部和东部以及俄克拉何马州东部,使用空气动力学替代表面被动采样器收集了气态氧化汞(GOM)干沉降测量数据。本研究的目的是初步描述得克萨斯州中部和东部环境GOM干沉降的量级和空间范围,为期12个月,其中包含降水总量、温度和风速的统计年均结果。研究目标是调查受燃煤公用事业锅炉排放影响的得克萨斯州地区的GOM干沉降,并将其与之前在俄克拉何马州东部和四角地区观测到的GOM干沉降测量结果进行比较。得克萨斯州的年度GOM干沉降速率估计值相对较低,在四个得克萨斯州监测点范围为0.1至0.3 ng/m²·h,与俄克拉何马州东部监测点记录的0.2 ng/m²·h的年度GOM干沉降速率估计值相似。得克萨斯州和俄克拉何马州东部的年度GOM干沉降速率估计值至少比之前在四角地区较为干旱的毗邻西部州新墨西哥州和科罗拉多州测量到的最高年度GOM干沉降速率估计值低四倍。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/3751ee7c931f/TSWJ2014-580723.005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/664c4c39cf6a/TSWJ2014-580723.001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/ddc1d4b6e308/TSWJ2014-580723.002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/d9031ff92796/TSWJ2014-580723.003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/4bcabbd5e0b1/TSWJ2014-580723.004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/3751ee7c931f/TSWJ2014-580723.005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/664c4c39cf6a/TSWJ2014-580723.001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/ddc1d4b6e308/TSWJ2014-580723.002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/d9031ff92796/TSWJ2014-580723.003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/4bcabbd5e0b1/TSWJ2014-580723.004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c458/3997905/3751ee7c931f/TSWJ2014-580723.005.jpg

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An application of passive samplers to understand atmospheric mercury concentration and dry deposition spatial distributions.应用被动采样器了解大气汞浓度和干沉降的空间分布。
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Testing the use of passive sampling systems for understanding air mercury concentrations and dry deposition across Florida, USA.
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J Air Waste Manag Assoc. 2012 Jan;62(1):52-63. doi: 10.1080/10473289.2011.622066.
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