利用阿秒时间分辨光电子能谱监测分子中电子波包的产生。
Monitoring the birth of an electronic wavepacket in a molecule with attosecond time-resolved photoelectron spectroscopy.
作者信息
Perveaux Aurelie, Lauvergnat David, Gatti Fabien, Halász Gábor J, Vibók Ágnes, Lasorne Benjamin
机构信息
Institut Charles Gerhardt, CNRS, Université Montpellier 2 , F-34095 Montpellier, France.
出版信息
J Phys Chem A. 2014 Sep 25;118(38):8773-8. doi: 10.1021/jp508218n. Epub 2014 Sep 8.
PMID:25167166
Abstract
Numerical simulations are presented to validate the possible use of cutting-edge attosecond time-resolved photoelectron spectroscopy to observe in real time the creation of an electronic wavepacket and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few femtoseconds.
摘要
本文进行了数值模拟，以验证前沿的阿秒时间分辨光电子能谱是否有可能实时观测到在紫外泵浦脉冲激发的中性分子中，在几飞秒内电子波包的产生以及随后的电子运动。
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