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双色旋转噪声谱和涨落相关揭示了量子点中的均匀线宽。

Two-colour spin noise spectroscopy and fluctuation correlations reveal homogeneous linewidths within quantum-dot ensembles.

机构信息

National High Magnetic Field Laboratory, Los Alamos, New Mexico 87545, USA.

Experimentelle Physik 2, Technische Universität Dortmund, D-44227 Dortmund, Germany.

出版信息

Nat Commun. 2014 Sep 15;5:4949. doi: 10.1038/ncomms5949.

Abstract

'Spin noise spectroscopy' is an optical technique for probing electron and hole spin dynamics that is based on detecting their intrinsic fluctuations while in thermal equilibrium. Here we show that fluctuation correlations can be further exploited in multi-probe noise studies to reveal information that in general cannot be accessed by conventional linear optical spectroscopy, such as the underlying homogeneous linewidths of individual constituents within inhomogeneously broadened systems. This is demonstrated in singly charged (In,Ga)As quantum-dot ensembles using two weak probe lasers: When the lasers have similar wavelengths, they probe the same quantum dots in the ensemble and show correlated spin fluctuations. In contrast, mutually detuned probe lasers measure different subsets of quantum dots, giving uncorrelated fluctuations. The noise correlation versus laser detuning directly reveals the quantum dot homogeneous linewidth even in the presence of a strong inhomogeneous broadening. Such noise-based correlation techniques are not limited to semiconductor spin systems, but are applicable to any system with measurable intrinsic fluctuations.

摘要

“自旋噪声光谱学”是一种探测电子和空穴自旋动力学的光学技术,它基于在热平衡时探测其固有涨落。在这里,我们表明,在多探针噪声研究中,可以进一步利用涨落相关来揭示通常无法通过传统线性光学光谱学获得的信息,例如非均匀展宽系统中各个组成部分的基本均匀线宽。这在使用两个弱探测激光的单电荷(In,Ga)As 量子点中得到了证明:当激光具有相似的波长时,它们探测到同一量子点中的相同量子点,并显示出相关的自旋涨落。相比之下,相互失谐的探测激光测量不同子集的量子点,给出不相关的涨落。噪声相关性与激光失谐的关系直接揭示了量子点的均匀线宽,即使在存在强非均匀展宽的情况下也是如此。这种基于噪声的相关技术不仅限于半导体自旋系统,而且适用于任何具有可测量固有涨落的系统。

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