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中国表层土壤中的多环芳烃:存在与分布

Polycyclic aromatic hydrocarbons in Chinese surface soil: occurrence and distribution.

作者信息

Ma Wan-Li, Liu Li-Yan, Tian Chong-Guo, Qi Hong, Jia Hong-Liang, Song Wei-Wei, Li Yi-Fan

机构信息

International Joint Research Center for Persistent Toxic Substances (IJRC-PTS), State Key Laboratory of Urban Water Resource and Environment, School of Municipal and Environmental Engineering, Harbin Institute of Technology, 202 Haihe Road, Nangang District, Harbin, 150090, Heilongjiang, China.

出版信息

Environ Sci Pollut Res Int. 2015 Mar;22(6):4190-200. doi: 10.1007/s11356-014-3648-3. Epub 2014 Oct 4.

Abstract

In this study, 16 polycyclic aromatic hydrocarbons (PAHs) were analyzed in 157 concurrently collected soil samples in 2005 over China. Higher concentration of ∑16PAHs was found in urban soil, followed by rural and background soil. The results indicated that PAHs in Chinese surface soil showed a primary distribution pattern, which was confirmed by the positive correlation with emission inventory. Based on the results of literature over the past 10 years (2004-2013) in China, the spatial distribution of PAHs in urban and rural soil was established. An obvious geographical distribution with PAH concentration was found, as higher in Eastern China and lower in Middle and Western China. Furthermore, PAH pollution in Chinese riverbank soil was summarized and showed higher levels, indicating their potential sources from polluted rivers. According to our knowledge, this is the first time to comprehensively study the PAH pollution status in Chinese surface soil on the national scale based on monitoring results.

摘要

本研究于2005年对中国同时采集的157份土壤样品中的16种多环芳烃(PAHs)进行了分析。城市土壤中∑16PAHs浓度较高,其次是农村土壤和背景土壤。结果表明,中国表层土壤中的PAHs呈现出主要分布模式,这一点通过与排放清单的正相关得到了证实。基于中国过去10年(2004 - 2013年)的文献结果,确定了城市和农村土壤中PAHs的空间分布。发现PAH浓度存在明显的地理分布,中国东部地区较高,中西部地区较低。此外,对中国河岸土壤中的PAH污染进行了总结,结果显示污染水平较高,表明其潜在来源为受污染的河流。据我们所知,这是首次基于监测结果在全国范围内全面研究中国表层土壤中的PAH污染状况。

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