Coppolaro V, Papi N, Khanbekyan A, Marinelli C, Mariotti E, Marmugi L, Moi L, Corradi L, Dainelli A, Arikawa H, Ishikawa T, Sakemi Y, Calabrese R, Mazzocca G, Tomassetti L, Ricci L
DSFTA and CNISM, University of Siena, via Roma 56, 53100 Siena, Italy.
INFN - Laboratori Nazionali di Legnaro, viale dell'Università 2, 35020 Legnaro (PD), Italy.
J Chem Phys. 2014 Oct 7;141(13):134201. doi: 10.1063/1.4896609.
We present here the first evidence of photodesorption induced by low-intensity non-resonant light from an yttrium thin foil, which works as a neutralizer for Rb and Fr ions beam. Neutral atoms are suddenly ejected from the metal surface in a pulsed regime upon illumination with a broadband flash light and then released in the free volume of a pyrex cells. Here atoms are captured by a Magneto-Optical Trap (MOT), which is effectively loaded by the photodesorption. Loading times of the order of the flash rise time are measured. Desorption is also obtained in the continuous regime, by exploiting CW visible illumination of the metallic neutralizer surface. We demonstrate that at lower CW light intensities vacuum conditions are not perturbed by the photodesorption and hence the MOT dynamics remains unaffected, while the trap population increases thanks to the incoming desorbed atoms flux. Even with the Y foil at room temperature and hence with no trapped atoms, upon visible illumination, the number of trapped atoms reaches 10(5). The experimental data are then analyzed by means of an analytical rate equation model, which allows the analysis of this phenomenon and its dynamics and allows the determination of critical experimental parameters and the test of the procedure in the framework of radioactive Francium trapping. In this view, together with an extensive investigation of the phenomenon with (85)Rb, the first demonstration of the photodesorption-aided loading of a (210)Fr MOT is shown.
我们在此展示了由钇薄箔发出的低强度非共振光诱导的光解吸的首个证据,该钇薄箔用作铷和钫离子束的中和器。在用宽带闪光灯照射时,中性原子以脉冲形式突然从金属表面喷射出来,然后释放到派热克斯玻璃细胞的自由空间中。在这里,原子被磁光阱(MOT)捕获,磁光阱通过光解吸有效地加载。测量了与闪光上升时间量级相当的加载时间。通过利用金属中和器表面的连续可见光照,在连续模式下也能实现解吸。我们证明,在较低的连续光强度下,真空条件不会因光解吸而受到干扰,因此磁光阱的动力学不受影响,而由于入射的解吸原子通量,阱中的原子数增加。即使钇箔处于室温且因此没有捕获原子,在可见光照射下,捕获的原子数也能达到10⁵ 。然后通过一个解析速率方程模型对实验数据进行分析,该模型能够分析这种现象及其动力学,确定关键实验参数,并在放射性钫捕获的框架内对该过程进行测试。从这个角度来看,连同对用⁸⁵Rb进行的该现象的广泛研究一起,展示了对²¹⁰Fr磁光阱光解吸辅助加载的首次证明。