Carlsbad Environmental Monitoring & Research Center, 1400 University Drive, Carlsbad, New Mexico 88220, United States.
Environ Sci Technol. 2014 Nov 4;48(21):12698-705. doi: 10.1021/es503649y. Epub 2014 Oct 24.
Recent incidents at the nation's only operating deep geologic nuclear waste repository, the Waste Isolation Pilot Plant (WIPP), resulted in the release of americium and plutonium from one or more defense-related transuranic (TRU) waste containers into the environment. WIPP is a U.S. Department of Energy mined geologic repository that has been in operation since March, 1999. Over 85,000 m3 of waste in various vented payload containers have been emplaced in the repository. The primary radionuclides within the disposed waste are 239+240Pu and 241Am, which account for more than 99% of the total TRU radioactivity disposed and scheduled for disposal in the repository. For the first time in its 15 years of operation, there was an airborne radiation release from the WIPP at approximately 11:30 PM Mountain Standard Time (MST) on Friday, February 14, 2014. The radiation release was likely caused by a chemical reaction inside a TRU waste drum that contained nitrate salts and organic sorbent materials. In a recent news release, DOE announced that photos taken of the waste underground showed evidence of heat and gas pressure resulting in a deformed lid, in material expelled through that deformation, and in melted plastic and rubber and polyethylene in the vicinity of that drum. Recent entries into underground Panel 7 have confirmed that at least one waste drum containing a nitrate salt bearing waste stream from Los Alamos National Laboratory was breached underground and was the most likely source of the release. Further investigation is underway to determine if other containers contributed to the release. Air monitoring across the WIPP site intensified following the first reports of radiation detection underground to ascertain whether or not there were releases to the ground surface. Independent analytical results of air filters from sampling stations on and near the WIPP facility have been released by us at the Carlsbad Environmental Monitoring & Research Center and confirmed trace amounts of 241Am and 239+240Pu, at ratios reflecting the suspect waste stream. The highest activity detected offsite was 115.2 μBq/m3 for 241Am and 10.2 μBq/m3 for 239+240 Pu. These concentrations in air were very small, localized, and below any level of public health or environmental concern.
最近,美国唯一运行的深层地质核废料处置库——废物隔离试验工厂(WIPP)发生了一些事件,导致一个或多个与国防相关的超铀(TRU)废物容器中的镅和钚释放到环境中。WIPP 是美国能源部运营的一个矿山地质处置库,自 1999 年 3 月以来一直在运行。在该处置库中,已处置了 85000 多立方米的各种通风有效载荷容器中的废物。处置废物中的主要放射性核素是 239+240Pu 和 241Am,它们占处置和计划在处置库中处置的总 TRU 放射性的 99%以上。在其 15 年的运行历史中,WIPP 首次在 2014 年 2 月 14 日星期五晚上 11 点 30 分左右发生了空气辐射释放。辐射释放可能是由于一个含有硝酸盐盐和有机吸附材料的 TRU 废物桶内的化学反应引起的。在最近的新闻发布中,美国能源部宣布,对地下废物拍摄的照片显示有热和气压的证据,导致一个变形的盖子,以及通过该变形喷出的材料,以及附近的鼓状物融化的塑料和橡胶以及聚乙烯。最近进入地下 7 号面板的记录证实,至少有一个装有洛斯阿拉莫斯国家实验室含硝酸盐盐的废物桶在地下破裂,是此次释放的最有可能的来源。正在进行进一步的调查,以确定是否有其他容器对此次释放做出了贡献。在地下首次报告检测到辐射后,WIPP 现场的空气监测加强,以确定是否有释放到地面。我们在卡尔斯巴德环境监测和研究中心公布了来自 WIPP 设施附近和附近采样站的空气过滤器的独立分析结果,证实了痕量的 241Am 和 239+240Pu,其比值反映了可疑的废物流。检测到的场外最高活性为 241Am 的 115.2 μBq/m3 和 239+240 Pu 的 10.2 μBq/m3。这些空气中的浓度非常小,局部,低于任何公共健康或环境关注的水平。