Liu Wei-Sheng, Tseng Hsin-Lun, Kuo Po-Chen
Opt Express. 2014 Aug 11;22(16):18860-9. doi: 10.1364/OE.22.018860.
In this study, the optical properties of InAs quantum dots (QDs) with various strain-reducing layers (SRLs) of GaAsSb and InGaAsSb are characterized using photoluminescence (PL) and time-resolved PL (TRPL) measurements. The room-temperature PL results for the InAs/InGaAsSb QDs revealed stronger emission intensities than InAs QDs capped with an GaAs(1-x)Sb(x) (x = 20%)SRL, although both samples were grown under the same Sb flux during the molecular beam epitaxy process. The InAs/InGaAsSb QDs showed a significant elongation of emission wavelengths to 1450 and 1310 nm for the ground and first-excited state at room temperature. The energy band alignment of the InAs QD heterostructures was found tailoring from type II to type I as the GaAsSb SRL was replaced by InGaAsSb layer, which improved the radiative efficiency and was verified by power-dependent PL and TRPL measurements. Post-growth rapid thermal annealing was applied on the InAs/InGaAsSb QDs to further enhance the QD quality and PL emission efficiency. The greatly improved PL intensity, reduced linewidth, shortened radiative lifetime, with increasing annealing temperature were demonstrated, and InAs/InGaAsSb QDs exhibited enhanced optical characteristics for long-wavelength emission applications.
在本研究中,利用光致发光(PL)和时间分辨光致发光(TRPL)测量对具有各种GaAsSb和InGaAsSb应变减少层(SRL)的InAs量子点(QD)的光学性质进行了表征。InAs/InGaAsSb量子点的室温PL结果显示,其发射强度比覆盖有GaAs(1-x)Sb(x)(x = 20%)SRL的InAs量子点更强,尽管这两个样品在分子束外延过程中是在相同的Sb通量下生长的。InAs/InGaAsSb量子点在室温下基态和第一激发态的发射波长显著延长至1450和1310 nm。随着GaAsSb SRL被InGaAsSb层取代,发现InAs量子点异质结构的能带排列从II型调整为I型,这提高了辐射效率,并通过功率相关的PL和TRPL测量得到了验证。对InAs/InGaAsSb量子点进行生长后快速热退火,以进一步提高量子点质量和PL发射效率。结果表明,随着退火温度的升高,PL强度大大提高,线宽减小,辐射寿命缩短,并且InAs/InGaAsSb量子点在长波长发射应用中表现出增强的光学特性。