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BaPb(1-x)Bi(x)O₃中无序驱动的金属-绝缘体转变及无无序临界温度的推断

Disorder driven metal-insulator transition in BaPb(1-x)Bi(x)O₃ and inference of disorder-free critical temperature.

作者信息

Luna Katherine, Giraldo-Gallo Paula, Geballe Theodore, Fisher Ian, Beasley Malcolm

机构信息

Department of Physics, Stanford University, Stanford, California 94305-4045, USA.

出版信息

Phys Rev Lett. 2014 Oct 24;113(17):177004. doi: 10.1103/PhysRevLett.113.177004. Epub 2014 Oct 21.

Abstract

We performed point-contact spectroscopy tunneling measurements on single crystal BaPb(1-x)Bi(x)O(3) for 0≤x≤0.28 at temperatures T=2-40  K and find a suppression in the density of states at low bias voltages that is characteristic of disordered metals. Both the correlation gap and the zero-temperature conductivity are zero at a critical concentration x(c)=0.30. Not only does this suggests that a disorder driven metal-insulator transition occurs before the onset of the charge disproportionated charge density wave insulator, but we also explore whether a scaling theory is applicable. In addition, we estimate the disorder-free critical temperature and compare these results to Ba(1-x)K(x)BiO(3).

摘要

我们在温度T = 2 - 40 K下对0≤x≤0.28的单晶BaPb(1 - x)Bi(x)O(3)进行了点接触光谱隧穿测量,发现在低偏置电压下态密度受到抑制,这是无序金属的特征。在临界浓度x(c)=0.30时,关联能隙和零温电导率均为零。这不仅表明在电荷 disproportionated 电荷密度波绝缘体出现之前发生了无序驱动的金属 - 绝缘体转变,而且我们还探讨了标度理论是否适用。此外,我们估计了无无序临界温度,并将这些结果与Ba(1 - x)K(x)BiO(3)进行了比较。

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