Parra Carolina, Niestemski Francis C, Contryman Alex W, Giraldo-Gallo Paula, Geballe Theodore H, Fisher Ian R, Manoharan Hari C
SLAC National Accelerator Laboratory, Stanford Institute for Materials and Energy Sciences, Menlo Park, CA 94025;
Department of Physics, Stanford University, Stanford, CA 94305.
Proc Natl Acad Sci U S A. 2021 Apr 20;118(16). doi: 10.1073/pnas.2017810118.
Spatial disorder has been shown to drive two-dimensional (2D) superconductors to an insulating phase through a superconductor-insulator transition (SIT). Numerical calculations predict that with increasing disorder, emergent electronic granularity is expected in these materials-a phenomenon where superconducting (SC) domains on the scale of the material's coherence length are embedded in an insulating matrix and coherently coupled by Josephson tunneling. Here, we present spatially resolved scanning tunneling spectroscopy (STS) measurements of the three-dimensional (3D) superconductor BaPb Bi O (BPBO), which surprisingly demonstrate three key signatures of emergent electronic granularity, having only been previously conjectured and observed in 2D thin-film systems. These signatures include the observation of emergent SC domains on the scale of the coherence length, finite energy gap over all space, and strong enhancement of spatial anticorrelation between pairing amplitude and gap magnitude as the SIT is approached. These observations are suggestive of 2D SC behavior embedded within a conventional 3D -wave host, an intriguing but still unexplained interdimensional phenomenon, which has been hinted at by previous experiments in which critical scaling exponents in the vicinity of a putative 3D quantum phase transition are consistent only with dimensionality = 2.
空间无序已被证明会通过超导体 - 绝缘体转变(SIT)将二维(2D)超导体驱动到绝缘相。数值计算预测,随着无序度增加,这些材料中会出现电子粒度现象——在这种现象中,材料相干长度尺度上的超导(SC)畴嵌入绝缘基质中,并通过约瑟夫森隧穿相干耦合。在此,我们展示了对三维(3D)超导体BaPbBiO(BPBO)的空间分辨扫描隧道谱(STS)测量,令人惊讶的是,这些测量展示了电子粒度出现的三个关键特征,此前仅在二维薄膜系统中被推测和观察到。这些特征包括在相干长度尺度上观察到出现的SC畴、整个空间的有限能隙,以及在接近SIT时配对幅度和能隙大小之间空间反相关的强烈增强。这些观察结果表明,在传统的三维波主体中嵌入了二维超导行为,这是一种有趣但仍未得到解释的跨维度现象,此前的实验曾暗示过这一现象,在这些实验中,假定的三维量子相变附近的临界标度指数仅与维度d = 2一致。