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种子自由电子激光器产生的多色脉冲:迈向非线性芯能级相干光谱学的发展

Multi-colour pulses from seeded free-electron-lasers: towards the development of non-linear core-level coherent spectroscopies.

作者信息

Bencivenga Filippo, Capotondi Flavio, Casolari Francesco, Dallari Francesco, Danailov Miltcho B, De Ninno Giovanni, Fausti Daniele, Kiskinova Maya, Manfredda Michele, Masciovecchio Claudio, Pedersoli Emanuele

机构信息

Elettra-Sincrotrone Trieste S.C.p.A., S.S. 14 km 163,5 in AREA Science Park, I-34149, Basovizza, Trieste, Italy.

出版信息

Faraday Discuss. 2014;171:487-503. doi: 10.1039/c4fd00100a. Epub 2014 Aug 13.

DOI:10.1039/c4fd00100a
PMID:25415809
Abstract

We report on new opportunities for ultrafast science thanks to the use of two-colour extreme ultraviolet (XUV) pulses at the FERMI free electron laser (FEL) facility. The two pulses have been employed to carry out a pioneering FEL-pump/FEL-probe diffraction experiment using a Ti target and tuning the FEL pulses to the M(2/3)-edge in order to explore the dependence of the dielectric constant on the excitation fluence. The future impact that the use of such a two-colour FEL emission will have on the development of ultrafast wave-mixing methods in the XUV/soft X-ray range is addressed and discussed.

摘要

我们报告了在费米自由电子激光(FEL)设施中使用双色极紫外(XUV)脉冲为超快科学带来的新机遇。这两个脉冲已被用于使用钛靶开展开创性的FEL泵浦/FEL探测衍射实验,并将FEL脉冲调谐到M(2/3)边缘,以探索介电常数对激发通量的依赖性。本文探讨并讨论了这种双色FEL发射在XUV/软X射线范围内对超快波混频方法发展的未来影响。

相似文献

1
Multi-colour pulses from seeded free-electron-lasers: towards the development of non-linear core-level coherent spectroscopies.种子自由电子激光器产生的多色脉冲:迈向非线性芯能级相干光谱学的发展
Faraday Discuss. 2014;171:487-503. doi: 10.1039/c4fd00100a. Epub 2014 Aug 13.
2
Invited article: Coherent imaging using seeded free-electron laser pulses with variable polarization: first results and research opportunities.特邀文章:使用具有可变偏振的种子自由电子激光脉冲的相干成像:初步结果与研究机遇
Rev Sci Instrum. 2013 May;84(5):051301. doi: 10.1063/1.4807157.
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Spectrotemporal shaping of seeded free-electron laser pulses.种子自由电子激光脉冲的光谱时间整形
Phys Rev Lett. 2015 Sep 11;115(11):114801. doi: 10.1103/PhysRevLett.115.114801. Epub 2015 Sep 8.
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Temporal cross-correlation of x-ray free electron and optical lasers using soft x-ray pulse induced transient reflectivity.利用软X射线脉冲诱导瞬态反射率对X射线自由电子激光与光学激光进行时间互相关分析。
Opt Express. 2012 May 7;20(10):11396-406. doi: 10.1364/OE.20.011396.
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Towards jitter-free pump-probe measurements at seeded free electron laser facilities.迈向种子自由电子激光装置下无抖动的泵浦-探测测量。
Opt Express. 2014 Jun 2;22(11):12869-79. doi: 10.1364/OE.22.012869.
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In situ single-shot diffractive fluence mapping for X-ray free-electron laser pulses.基于单幅记录的 X 射线自由电子激光脉冲漫衍函数实时测量
Nat Commun. 2018 Jan 15;9(1):214. doi: 10.1038/s41467-017-02567-0.
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Single-shot spectro-temporal characterization of XUV pulses from a seeded free-electron laser.对种子自由电子激光产生的极紫外脉冲进行单次光谱-时间特性表征。
Nat Commun. 2015 Aug 20;6:8075. doi: 10.1038/ncomms9075.
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Four-wave-mixing experiments with seeded free electron lasers.基于种子自由电子激光的四波混频实验。
Faraday Discuss. 2016 Dec 16;194:283-303. doi: 10.1039/c6fd00089d.
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A setup for resonant inelastic soft x-ray scattering on liquids at free electron laser light sources.一种用于在自由电子激光光源下对液体进行共振非弹性软X射线散射的装置。
Rev Sci Instrum. 2012 Dec;83(12):123109. doi: 10.1063/1.4772685.
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Development of a multipurpose vacuum chamber for serial optical and diffraction experiments with free electron laser radiation.用于自由电子激光辐射的系列光学和衍射实验的多功能真空腔的研制。
Rev Sci Instrum. 2010 Apr;81(4):045105. doi: 10.1063/1.3327816.

引用本文的文献

1
Perspective: Opportunities for ultrafast science at SwissFEL.观点:瑞士自由电子激光装置助力超快科学发展的机遇
Struct Dyn. 2018 Jan 8;4(6):061602. doi: 10.1063/1.4997222. eCollection 2017 Nov.
2
Time-resolved X-ray spectroscopies of chemical systems: New perspectives.时间分辨 X 射线光谱学在化学体系中的应用:新视角。
Struct Dyn. 2016 May 31;3(3):031001. doi: 10.1063/1.4953104. eCollection 2016 May.
3
Widely tunable two-colour seeded free-electron laser source for resonant-pump resonant-probe magnetic scattering.用于共振泵浦共振探测磁散射的宽可调谐双色种子自由电子激光源。
Nat Commun. 2016 Jan 13;7:10343. doi: 10.1038/ncomms10343.
4
Four-wave mixing experiments with extreme ultraviolet transient gratings.利用极紫外瞬态光栅进行的四波混频实验。
Nature. 2015 Apr 9;520(7546):205-8. doi: 10.1038/nature14341.