Clarke Lorraine Weller, Jenerette G Darrel, Bain Daniel J
Department of Botany and Plant Sciences, University of California, Riverside, CA 92521, USA.
Department of Geology and Planetary Science, University of Pittsburgh, Pittsburgh, PA 15260, USA.
Environ Pollut. 2015 Feb;197:1-12. doi: 10.1016/j.envpol.2014.11.015. Epub 2014 Nov 29.
Heavy metals in urban soils can compromise human health, especially in urban gardens, where gardeners may ingest contaminated dust or crops. To identify patterns of urban garden metal contamination, we measured concentrations and bioavailability of Pb, As, and Cd in soils associated with twelve community gardens in Los Angeles County, CA. This included sequential extractions to partition metals among exchangeable, reducible, organic, or residual fractions. Proximity to road increased all metal concentrations, suggesting vehicle emissions sources. Reducible Pb increased with neighborhood age, suggesting leaded paint as a likely pollutant source. Exchangeable Cd and As both increased with road proximity. Only cultivated soils showed an increase in exchangeable As with road proximity, potentially due to reducing humic acid interactions while Cd bioavailability was mitigated by organic matter. Understanding the geochemical phases and metal bioavailability allows incorporation of contamination patterns into urban planning.
城市土壤中的重金属会危害人体健康,尤其是在城市花园中,园丁可能会摄入受污染的灰尘或作物。为了确定城市花园金属污染的模式,我们测量了加利福尼亚州洛杉矶县12个社区花园土壤中铅、砷和镉的浓度及生物有效性。这包括连续提取,以将金属分配到可交换、可还原、有机或残留部分。靠近道路会增加所有金属的浓度,表明车辆排放是污染源。可还原铅随着社区年限的增加而增加,表明含铅油漆可能是污染物来源。可交换镉和砷都随着与道路距离的缩短而增加。只有耕种土壤中可交换砷随着与道路距离的缩短而增加,这可能是由于腐殖酸相互作用减少,而镉的生物有效性则因有机物而降低。了解地球化学相和金属生物有效性有助于将污染模式纳入城市规划。