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中国北京一个典型居民区的环境细颗粒物(PM2.5)及其相关金属的浓度与季节变化

Concentrations and seasonal variation of ambient PM(2.5) and associated metals at a typical residential area in Beijing, China.

作者信息

Yang Jing, Fu Qiang, Guo Xiaoshuang, Chu Baolin, Yao Yawei, Teng Yanguo, Wang Yeyao

机构信息

College of Water Sciences, Beijing Normal University, No. 19, XinJieKouWai St., HaiDian District, Beijing, 100875, People's Republic of China.

出版信息

Bull Environ Contam Toxicol. 2015 Feb;94(2):232-9. doi: 10.1007/s00128-014-1443-y. Epub 2014 Dec 21.

DOI:10.1007/s00128-014-1443-y
PMID:25528273
Abstract

In this study, continuous monitoring of PM2.5 was carried out for 1 year period at one of the largest residential areas in Beijing. Annual mean of PM2.5 during sampling period was 100.4 µg/m(3). The seasonal variation trend of PM2.5 was winter > spring > autumn and summer. The total mass concentrations of metals in PM2.5 ranged from 0.4 to 13.2 μg/m(3). There were significant (p < 0.05) seasonal variations for concentrations of Ca, Al, Mn, As, Rb, Cr, Ni, Cd and Co, seasonal variations in PM-associated metals were not necessarily the same as the seasonal variation in PM2.5, related to differing seasonal trends in source types. The impact of meteorological factors (e.g., wind speed) on metals levels of PM2.5 was found to be significant by regression models. The EFs value of Ag, Ca, Cd, Pb, Zn, As, Cu, and Cr were higher than ten, suggesting that those elements were primarily contributed by anthropogenic sources. Seasonal characteristic of EFs were found for As, Cr, Ca and Ag, which indicating the seasonal pollution sources types for those metals. Overall, these findings indicated that the pollution control of ambient PM2.5 should not be negligible in residential area in Beijing and the local government should pertinent and accurate prevent and control of air pollution as well as protect human health.

摘要

在本研究中,对北京最大的居民区之一进行了为期1年的PM2.5连续监测。采样期间PM2.5的年平均值为100.4µg/m³。PM2.5的季节变化趋势为冬季>春季>秋季和夏季。PM2.5中金属的总质量浓度范围为0.4至13.2µg/m³。Ca、Al、Mn、As、Rb、Cr、Ni、Cd和Co的浓度存在显著(p<0.05)季节变化,与颗粒物相关的金属的季节变化不一定与PM2.5的季节变化相同,这与源类型的不同季节趋势有关。通过回归模型发现气象因素(如风速)对PM2.5中金属含量的影响显著。Ag、Ca、Cd、Pb、Zn、As、Cu和Cr的富集因子值高于10,表明这些元素主要来自人为源。发现As、Cr、Ca和Ag的富集因子具有季节特征,这表明了这些金属的季节性污染源类型。总体而言,这些发现表明,北京居民区环境PM2.5的污染控制不容忽视,地方政府应针对性地、准确地预防和控制空气污染,保护人类健康。

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