Drezet A, Sonnefraud Y, Cuche A, Mollet O, Berthel M, Huant S
Université Grenoble Alpes, Institut NEEL, F-38000 Grenoble, France; CNRS, Institut NEEL, F-38042 Grenoble, France.
Université Grenoble Alpes, Institut NEEL, F-38000 Grenoble, France; CNRS, Institut NEEL, F-38042 Grenoble, France; CEMES CNRS UPR 8011, 29 rue J. Marvig, 31055 Toulouse Cedex 4, France.
Micron. 2015 Mar;70:55-63. doi: 10.1016/j.micron.2014.12.004. Epub 2014 Dec 26.
We review our recent developments of near-field scanning optical microscopy (NSOM) that uses an active tip made of a single fluorescent nanodiamond (ND) grafted onto the apex of a substrate fiber tip. The ND hosting a limited number of nitrogen-vacancy (NV) color centers, such a tip is a scanning quantum source of light. The method for preparing the ND-based tips and their basic properties are summarized. Then we discuss theoretically the concept of spatial resolution that is achievable in this special NSOM configuration and find it to be only limited by the scan height over the imaged system, in contrast with the standard aperture-tip NSOM whose resolution depends critically on both the scan height and aperture diameter. Finally, we describe a scheme we have introduced recently for high-resolution imaging of nanoplasmonic structures with ND-based tips that is capable of approaching the ultimate resolution anticipated by theory.
我们回顾了近场扫描光学显微镜(NSOM)的近期进展,该显微镜使用由单个荧光纳米金刚石(ND)制成的有源探针,该纳米金刚石嫁接到基底光纤探针的顶端。这种含有有限数量氮空位(NV)色心的ND探针是一种扫描量子光源。总结了基于ND的探针的制备方法及其基本特性。然后,我们从理论上讨论了在这种特殊的NSOM配置中可实现的空间分辨率概念,发现它仅受成像系统上方扫描高度的限制,这与标准孔径探针NSOM形成对比,后者的分辨率关键取决于扫描高度和孔径直径。最后,我们描述了一种最近引入的使用基于ND的探针进行纳米等离子体结构高分辨率成像的方案,该方案能够接近理论预期的极限分辨率。