文献检索文档翻译深度研究
Suppr Zotero 插件Zotero 插件
邀请有礼套餐&价格历史记录

新学期,新优惠

限时优惠:9月1日-9月22日

30天高级会员仅需29元

1天体验卡首发特惠仅需5.99元

了解详情
不再提醒
插件&应用
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
高级版
套餐订阅购买积分包
AI 工具
文献检索文档翻译深度研究
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2025

观察单层 MoSe2-WSe2 异质结构中的长寿命层间激子。

Observation of long-lived interlayer excitons in monolayer MoSe2-WSe2 heterostructures.

机构信息

Department of Physics, University of Washington, Seattle, Washington 98195, USA.

Department of Materials Science and Engineering, University of Washington, Seattle, Washington 98195, USA.

出版信息

Nat Commun. 2015 Feb 24;6:6242. doi: 10.1038/ncomms7242.


DOI:10.1038/ncomms7242
PMID:25708612
Abstract

Van der Waals bound heterostructures constructed with two-dimensional materials, such as graphene, boron nitride and transition metal dichalcogenides, have sparked wide interest in device physics and technologies at the two-dimensional limit. One highly coveted heterostructure is that of differing monolayer transition metal dichalcogenides with type-II band alignment, with bound electrons and holes localized in individual monolayers, that is, interlayer excitons. Here, we report the observation of interlayer excitons in monolayer MoSe2-WSe2 heterostructures by photoluminescence and photoluminescence excitation spectroscopy. We find that their energy and luminescence intensity are highly tunable by an applied vertical gate voltage. Moreover, we measure an interlayer exciton lifetime of ~1.8 ns, an order of magnitude longer than intralayer excitons in monolayers. Our work demonstrates optical pumping of interlayer electric polarization, which may provoke further exploration of interlayer exciton condensation, as well as new applications in two-dimensional lasers, light-emitting diodes and photovoltaic devices.

摘要

范德华异质结构由二维材料构建,如石墨烯、氮化硼和过渡金属二卤化物,在二维极限的器件物理和技术方面引起了广泛的兴趣。一种备受追捧的异质结是具有 II 型能带排列的不同单层过渡金属二卤化物,其束缚电子和空穴定域在单个单层中,即层间激子。在这里,我们通过光致发光和光致发光激发光谱报告了在单层 MoSe2-WSe2 异质结构中观察到的层间激子。我们发现它们的能量和发光强度可以通过施加的垂直栅极电压高度可调。此外,我们测量了~1.8 ns 的层间激子寿命,比单层中的层内激子长一个数量级。我们的工作证明了层间电极化的光泵浦,这可能会引发对层间激子凝聚的进一步探索,以及在二维激光、发光二极管和光伏器件中的新应用。

相似文献

[1]
Observation of long-lived interlayer excitons in monolayer MoSe2-WSe2 heterostructures.

Nat Commun. 2015-2-24

[2]
Probing the Interlayer Exciton Physics in a MoS/MoSe/MoS van der Waals Heterostructure.

Nano Lett. 2017-9-18

[3]
Probing Evolution of Twist-Angle-Dependent Interlayer Excitons in MoSe/WSe van der Waals Heterostructures.

ACS Nano. 2017-4-6

[4]
Long-Lived Direct and Indirect Interlayer Excitons in van der Waals Heterostructures.

Nano Lett. 2017-8-1

[5]
Interlayer Exciton Optoelectronics in a 2D Heterostructure p-n Junction.

Nano Lett. 2017-1-4

[6]
Interlayer Coupling and Gate-Tunable Excitons in Transition Metal Dichalcogenide Heterostructures.

Nano Lett. 2017-11-30

[7]
Interlayer Exciton-Phonon Coupling in MoSe/WSe Heterostructures.

Nano Lett. 2024-9-25

[8]
Valley-polarized exciton dynamics in a 2D semiconductor heterostructure.

Science. 2016-2-12

[9]
Double Indirect Interlayer Exciton in a MoSe/WSe van der Waals Heterostructure.

ACS Nano. 2018-5-22

[10]
Coupling Interlayer Excitons to Whispering Gallery Modes in van der Waals Heterostructures.

Nano Lett. 2020-8-12

引用本文的文献

[1]
Efficient energy transfer in a hybrid organic-inorganic van der Waals heterostructure.

Sci Adv. 2025-9-5

[2]
Enhanced Light Emission in MoSe-WSe Lateral Heterostructures in the Electron-Hole Plasma Regime.

J Phys Chem Lett. 2025-8-14

[3]
Influence of interface dielectric disorder on interlayer excitons in mixed binary/ternary TMD heterostructures.

Nanoscale Adv. 2025-7-25

[4]
Enhancing interlayer exciton dynamics by coupling with monolithic cavities via the field-induced Stark effect.

Nat Nanotechnol. 2025-7-17

[5]
Characterizing Interlayer Excitons by Spectral Signature in Scattering Visible Near-Field Microscopy.

J Phys Chem Lett. 2025-7-10

[6]
Engineering of MoSe and WSe Monolayers and Heterostructures by DFT-Molecular Dynamics Simulations.

ACS Appl Mater Interfaces. 2025-7-9

[7]
Highly Polarized Single-Photon Emission from Localized Excitons in a WSe/CrSBr Heterostructure.

ACS Photonics. 2025-5-29

[8]
Emergent 2D van der Waals materials photonic sources.

Nanophotonics. 2025-3-11

[9]
Possible evidence of excitonic condensation in a topological insulator.

Proc Natl Acad Sci U S A. 2025-5-6

[10]
Designable excitonic effects in van der Waals artificial crystals with exponentially growing thickness.

Nat Commun. 2025-3-19

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

推荐工具

医学文档翻译智能文献检索