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布朗动力学:从玻璃态到平凡态。

Brownian dynamics: from glassy to trivial.

作者信息

Jacquin Hugo, Kim Bongsoo, Kawasaki Kyozi, van Wijland Frédéric

机构信息

Laboratoire Matière et Systèmes Complexes, UMR 7057 CNRS/P7, Université Paris Diderot, 10 rue Alice Domon et Léonie Duquet, 75205 Paris cedex 13, France.

Department of Physics and Institute for Soft and Bio Matter Science, Changwon National University, Changwon 641-773, Korea.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Feb;91(2):022130. doi: 10.1103/PhysRevE.91.022130. Epub 2015 Feb 20.

Abstract

We endow a system of interacting particles with two distinct, local, Markovian, and reversible microscopic dynamics that both converge to the Boltzmann-Gibbs equilibrium of standard liquids. While the first, standard, one leads to glassy dynamics, we use field-theoretical techniques to show that the latter displays no sign of glassiness. The approximations we use, akin to the mode-coupling approximation, are famous for magnifying glassy aspects of the dynamics, supposedly through the neglect of activated events. Despite this, the modified dynamics seem to stick to standard liquid relaxation. This finding singles out as applying to a realistic system of interacting particles in low dimensions and questions the role of the dynamical rules used to explore a given static free-energy landscape. Moreover, our peculiar choice of dynamical rules offers the possibility of a direct connection with replica theory, and our findings therefore call for a clarification of the interplay between replica theory and the underlying dynamics of the system.

摘要

我们赋予一个相互作用粒子系统两种不同的、局部的、马尔可夫的且可逆的微观动力学,这两种动力学都收敛到标准液体的玻尔兹曼 - 吉布斯平衡态。虽然第一种标准动力学导致玻璃态动力学,但我们使用场论技术表明,后者没有显示出玻璃态的迹象。我们所使用的近似方法类似于模式耦合近似,以放大动力学中的玻璃态方面而闻名,据推测这是通过忽略活化事件实现的。尽管如此,修改后的动力学似乎仍遵循标准液体弛豫。这一发现适用于低维相互作用粒子的现实系统,并对用于探索给定静态自由能景观的动力学规则的作用提出了质疑。此外,我们对动力学规则的特殊选择提供了与副本理论直接联系的可能性,因此我们的发现要求澄清副本理论与系统底层动力学之间的相互作用。

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Brownian dynamics: from glassy to trivial.布朗动力学:从玻璃态到平凡态。
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