Tompkins Nathan, Cambria Matthew Carl, Wang Adam L, Heymann Michael, Fraden Seth
Physics Department, Brandeis University, Waltham, Massachusetts 02453, USA.
Chaos. 2015 Jun;25(6):064611. doi: 10.1063/1.4922056.
Methods for creating custom planar networks of diffusively coupled chemical oscillators and perturbing individual oscillators within the network are presented. The oscillators consist of the Belousov-Zhabotinsky (BZ) reaction contained in an emulsion. Networks of drops of the BZ reaction are created with either Dirichlet (constant-concentration) or Neumann (no-flux) boundary conditions in a custom planar configuration using programmable illumination for the perturbations. The differences between the observed network dynamics for each boundary condition are described. Using light, we demonstrate the ability to control the initial conditions of the network and to cause individual oscillators within the network to undergo sustained period elongation or a one-time phase delay.
本文介绍了创建扩散耦合化学振荡器的定制平面网络以及扰动网络中单个振荡器的方法。振荡器由乳液中包含的贝洛索夫 - 扎博廷斯基(BZ)反应组成。使用可编程照明进行扰动,在定制平面配置中创建具有狄利克雷(恒定浓度)或诺伊曼(无通量)边界条件的BZ反应液滴网络。描述了每种边界条件下观察到的网络动力学之间的差异。通过光,我们展示了控制网络初始条件以及使网络中的单个振荡器经历持续周期延长或一次性相位延迟的能力。