Frik Malgorzata, Fernández-Gallardo Jacob, Gonzalo Oscar, Mangas-Sanjuan Víctor, González-Alvarez Marta, Serrano del Valle Alfonso, Hu Chunhua, González-Alvarez Isabel, Bermejo Marival, Marzo Isabel, Contel María
†Department of Chemistry, Brooklyn College, The City University of New York, Brooklyn, New York 11210, United States.
‡Chemistry Ph.D. Program, The Graduate Center, The City University of New York, 365 Fifth Avenue, New York, New York 10016, United States.
J Med Chem. 2015 Aug 13;58(15):5825-41. doi: 10.1021/acs.jmedchem.5b00427. Epub 2015 Jul 22.
New organometallic gold(III) and platinum(II) complexes containing iminophosphorane ligands are described. Most of them are more cytotoxic to a number of human cancer cell lines than cisplatin. Cationic Pt(II) derivatives 4 and 5, which differ only in the anion, Hg2Cl6(2-) or PF6(-) respectively, display almost identical IC50 values in the sub-micromolar range (25-335-fold more active than cisplatin on these cell lines). The gold compounds induced mainly caspase-independent cell death, as previously reported for related cycloaurated compounds containing IM ligands. Cycloplatinated compounds 3, 4, and 5 can also activate alternative caspase-independent mechanisms of death. However, at short incubation times cell death seems to be mainly caspase dependent, suggesting that the main mechanism of cell death for these compounds is apoptosis. Mercury-free compound 5 does not interact with plasmid (pBR322) DNA or with calf thymus DNA. Permeability studies of 5 by two different assays, in vitro Caco-2 monolayers and a rat perfusion model, have revealed a high permeability profile for this compound (comparable to that of metoprolol or caffeine) and an estimated oral fraction absorbed of 100%, which potentially makes it a good candidate for oral administration.
本文描述了含有亚氨基膦烷配体的新型有机金属金(III)和铂(II)配合物。其中大多数对多种人类癌细胞系的细胞毒性比顺铂更强。阳离子铂(II)衍生物4和5仅在阴离子上有所不同,分别为Hg2Cl6(2-)或PF6(-),在亚微摩尔范围内显示出几乎相同的IC50值(在这些细胞系上比顺铂活性高25 - 335倍)。如先前报道的含IM配体的相关环金化合物一样,金化合物主要诱导不依赖半胱天冬酶的细胞死亡。环铂化合物3、4和5也能激活其他不依赖半胱天冬酶的死亡机制。然而,在短时间孵育时,细胞死亡似乎主要依赖半胱天冬酶,这表明这些化合物的主要细胞死亡机制是凋亡。无汞化合物5不与质粒(pBR322)DNA或小牛胸腺DNA相互作用。通过两种不同的测定方法,即体外Caco - 2单层细胞和大鼠灌注模型对5进行的通透性研究表明,该化合物具有高通透性特征(与美托洛尔或咖啡因相当),估计口服吸收分数为100%,这使其有可能成为口服给药的良好候选药物。