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Enthalpies of mixing of liquid ternary Co-Li-Sn alloys.

作者信息

Yakymovych Andriy, Fürtauer Siegfried, Flandorfer Hans, Ipser Herbert

机构信息

Department of Inorganic Chemistry (Materials Chemistry), University of Vienna, Vienna, Austria.

出版信息

Monatsh Chem. 2014;145(11):1697-1706. doi: 10.1007/s00706-014-1284-8. Epub 2014 Sep 24.

Abstract

ABSTRACT

The partial and integral molar enthalpies of mixing of liquid Co-Li-Sn alloys were determined using drop calorimetry. The investigations were performed along six sections by the addition of lithium to mixtures with the compositions [Formula: see text]/[Formula: see text] ≈ 2:98, [Formula: see text]/[Formula: see text] ≈ 1:9, and [Formula: see text]/[Formula: see text] ≈ 3:17 as well as by the addition of cobalt to mixtures with the compositions [Formula: see text]/[Formula: see text] ≈ 3:17, [Formula: see text]/[Formula: see text] ≈ 1:2, and [Formula: see text]/[Formula: see text] ≈ 1:1 at a temperature of 1,173 K. The Co-Li-Sn system shows exothermic behavior of the integral molar enthalpy of mixing in the investigated concentration range. The integral molar enthalpy of mixing of liquid Co-Li system was calculated by Miedema's model to fit our measured ternary data using an extended Redlich-Kister-Muggianu model for substitutional solutions.

摘要
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c2ea/4495026/7a7d41bdf933/706_2014_1284_Fig1_HTML.jpg

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