碳化滤纸负载的FeNi合金上生物质衍生分子的连续还原胺化反应
Continuous Reductive Amination of Biomass-Derived Molecules over Carbonized Filter Paper-Supported FeNi Alloy.
作者信息
Chieffi Gianpaolo, Braun Max, Esposito Davide
机构信息
Department of Colloid Chemistry, Max-Planck-Institute of Colloids and Interfaces, 14424, Potsdam, Germany.
出版信息
ChemSusChem. 2015 Nov;8(21):3590-4. doi: 10.1002/cssc.201500804. Epub 2015 Sep 18.
This paper reports the continuous reductive amination of different molecules, including biomass-related compounds, over carbon-supported FeNi nanoparticles obtained on the basis of inexpensive and abundant metal precursors and cellulose. A biorefinery case study for the preparation of pyrrolidones via acid-catalyzed hydrolysis of glucose followed by reductive amination of the obtained levulinic acid is described.
本文报道了在基于廉价且丰富的金属前驱体和纤维素制备的碳负载FeNi纳米颗粒上，对包括生物质相关化合物在内的不同分子进行连续还原胺化反应。文中描述了一个生物炼制案例研究，该研究通过葡萄糖的酸催化水解制备γ-戊内酯，然后将所得的乙酰丙酸进行还原胺化反应来制备吡咯烷酮。
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