School of Materials Science and Engineering, Georgia Institute of Technology , Atlanta, Georgia 30332, United States.
School of Electronic and Information Engineering, Beijing Jiaotong University , Beijing 100044, China.
ACS Nano. 2015 Nov 24;9(11):11056-63. doi: 10.1021/acsnano.5b04486. Epub 2015 Oct 26.
Micro total analysis system (μTAS) is one of the important tools for modern analytical sciences. In this paper, we not only propose the concept of integrating the self-powered triboelectric microfluidic nanosensor (TMN) with μTAS, but also demonstrate that the developed system can be used as an in situ tool to quantify the flowing liquid for microfluidics and solution chemistry. The TMN automatically generates electric outputs when the fluid passing through it and the outputs are affected by the solution temperature, polarity, ionic concentration, and fluid flow velocity. The self-powered TMN can detect the flowing water velocity, position, reaction temperature, ethanol, and salt concentrations. We also integrate the TMNs in a μTAS platform to directly characterize the synthesis of Au nanoparticles by a chemical reduction method.
微全分析系统(μTAS)是现代分析科学的重要工具之一。本文不仅提出了将自供电摩擦电微流控纳米传感器(TMN)与μTAS 集成的概念,而且还证明了所开发的系统可作为用于微流控和溶液化学的定量流动液体的原位工具。当流体流过 TMN 时,TMN 会自动产生电输出,而输出会受到溶液温度、极性、离子浓度和流体流速的影响。自供电 TMN 可以检测水流速度、位置、反应温度、乙醇和盐浓度。我们还将 TMNs 集成到 μTAS 平台中,以直接表征通过化学还原法合成的金纳米粒子。