Malerba Mario, Alabastri Alessandro, Miele Ermanno, Zilio Pierfrancesco, Patrini Maddalena, Bajoni Daniele, Messina Gabriele C, Dipalo Michele, Toma Andrea, Proietti Zaccaria Remo, De Angelis Francesco
Istituto Italiano di Tecnologia - Via Morego, 30, I-16163 Genova, Italy.
University of Pavia, Physics Department - Via Bassi, 6, I-27100 Pavia, Italy.
Sci Rep. 2015 Nov 10;5:16436. doi: 10.1038/srep16436.
The exploitation of surface plasmon polaritons has been mostly limited to the visible and near infrared range, due to the low frequency limit for coherent plasmon excitation and the reduction of confinement on the metal surface for lower energies. In this work we show that 3D--out of plane--nanostructures can considerably increase the intrinsic quality of the optical output, light confinement and electric field enhancement factors, also in the near and mid-infrared. We suggest that the physical principle relies on the combination of far field and near field interactions between neighboring antennas, promoted by the 3D out-of-plane geometry. We first analyze the changes in the optical behavior, which occur when passing from a single on-plane nanostructure to a 3D out-of-plane configuration. Then we show that by arranging the nanostructures in periodic arrays, 3D architectures can provide, in the mid-IR, a much stronger plasmonic response, compared to that achievable with the use of 2D configurations, leading to higher energy harvesting properties and improved Q-factors, with bright perspective up to the terahertz range.
由于相干等离子体激元激发的低频限制以及较低能量下金属表面限制的降低,表面等离激元极化激元的利用大多局限于可见光和近红外范围。在这项工作中,我们表明三维(平面外)纳米结构可以显著提高光学输出的内在质量、光限制和电场增强因子,在近红外和中红外波段也是如此。我们认为物理原理依赖于相邻天线之间远场和近场相互作用的结合,这是由三维平面外几何结构促成的。我们首先分析从单个平面内纳米结构转变为三维平面外结构时光学行为的变化。然后我们表明,通过将纳米结构排列成周期性阵列,与使用二维结构相比,三维结构在中红外波段可以提供更强的等离子体响应,从而带来更高的能量收集特性和改善的品质因数,在太赫兹范围内有着光明的前景。