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冰核活性粒子可通过降水云被有效去除。

Ice nucleation active particles are efficiently removed by precipitating clouds.

作者信息

Stopelli Emiliano, Conen Franz, Morris Cindy E, Herrmann Erik, Bukowiecki Nicolas, Alewell Christine

机构信息

Environmental Geosciences, University of Basel, CH-4056 Basel, Switzerland.

INRA, UR0407 Pathologie Végétale, F-84143 Montfavet cedex, France.

出版信息

Sci Rep. 2015 Nov 10;5:16433. doi: 10.1038/srep16433.

Abstract

Ice nucleation in cold clouds is a decisive step in the formation of rain and snow. Observations and modelling suggest that variations in the concentrations of ice nucleating particles (INPs) affect timing, location and amount of precipitation. A quantitative description of the abundance and variability of INPs is crucial to assess and predict their influence on precipitation. Here we used the hydrological indicator δ(18)O to derive the fraction of water vapour lost from precipitating clouds and correlated it with the abundance of INPs in freshly fallen snow. Results show that the number of INPs active at temperatures ≥ -10 °C (INPs-10) halves for every 10% of vapour lost through precipitation. Particles of similar size (>0.5 μm) halve in number for only every 20% of vapour lost, suggesting effective microphysical processing of INPs during precipitation. We show that INPs active at moderate supercooling are rapidly depleted by precipitating clouds, limiting their impact on subsequent rainfall development in time and space.

摘要

冷云中的冰核形成是雨雪形成过程中的决定性步骤。观测和模型表明,冰核粒子(INPs)浓度的变化会影响降水的时间、地点和降水量。对INPs丰度和变异性进行定量描述对于评估和预测它们对降水的影响至关重要。在这里,我们使用水文指标δ(18)O来推导降水云中损失的水汽比例,并将其与新降雪中INPs的丰度相关联。结果表明,在温度≥ -10°C时具有活性的INPs数量(INPs-10)每因降水损失10%的水汽就减半。类似大小(>0.5μm)的粒子数量每因降水损失20%的水汽才减半,这表明降水过程中INPs发生了有效的微物理过程。我们表明,在适度过冷状态下具有活性的INPs会被降水云迅速消耗,从而在时间和空间上限制了它们对后续降雨发展的影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2d9e/4639768/507520b872eb/srep16433-f1.jpg

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