CIC nanoGUNE , 20018 Donostia - San Sebastián, Spain.
Centro de Fisica de Materiales CSIC-UPV/EHU and Donostia International Physics Center DIPC , 20018 Donostia - San Sebastián, Spain.
Nano Lett. 2016 Jan 13;16(1):663-70. doi: 10.1021/acs.nanolett.5b04416. Epub 2015 Dec 14.
Chiral antennas and metasurfaces can be designed to react differently to left- and right-handed circularly polarized light, which enables novel optical properties such as giant optical activity and negative refraction. Here, we demonstrate that the underlying chiral near-field distributions can be directly mapped with scattering-type scanning near-field optical microscopy employing circularly polarized illumination. We apply our technique to visualize, for the first time, the circular-polarization selective nanofocusing of infrared light in Archimedean spiral antennas, and explain this chiral optical effect by directional launching of traveling waves in analogy to antenna theory. Moreover, we near-field image single-layer rosette and asymmetric dipole-monopole metasurfaces and find negligible and strong chiral optical near-field contrast, respectively. Our technique paves the way for near-field characterization of optical chirality in metal nanostructures, which will be essential for the future development of chiral antennas and metasurfaces and their applications.
手性天线和超表面可以设计为对左旋和右旋圆偏振光产生不同的反应,从而产生巨大的旋光性和负折射等新颖的光学性质。在这里,我们证明可以通过采用圆偏振光照明的散射型扫描近场光学显微镜直接映射其手性近场分布。我们首次应用该技术可视化阿基米德螺旋天线中红外光的圆偏振选择性纳米聚焦,并通过类似于天线理论的行波定向发射来解释这种手性光学效应。此外,我们近场成像单层蔷薇花和非对称偶极单极超表面,并分别发现可以忽略和强烈的手性光学近场对比度。我们的技术为金属纳米结构中光学手性的近场表征铺平了道路,这对于手性天线和超表面及其应用的未来发展至关重要。