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随机薄膜去湿的完全非线性动力学

Fully nonlinear dynamics of stochastic thin-film dewetting.

作者信息

Nesic S, Cuerno R, Moro E, Kondic L

机构信息

Departamento de Matemáticas & Grupo Interdisciplinar de Sistemas Complejos (GISC), Universidad Carlos III de Madrid, 28911 Leganés, Spain.

Department of Mathematical Sciences, New Jersey Institute of Technology, Newark, New Jersey, USA.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Dec;92(6):061002. doi: 10.1103/PhysRevE.92.061002. Epub 2015 Dec 3.

Abstract

The spontaneous formation of droplets via dewetting of a thin fluid film from a solid substrate allows materials nanostructuring. Often, it is crucial to be able to control the evolution, and to produce patterns characterized by regularly spaced droplets. While thermal fluctuations are expected to play a role in the dewetting process, their relevance has remained poorly understood, particularly during the nonlinear stages of evolution that involve droplet formation. Within a stochastic lubrication framework, we show that thermal noise substantially influences the process of droplets formation. Stochastic systems feature a smaller number of droplets with a larger variability in size and space distribution, when compared to their deterministic counterparts. Finally, we discuss the influence of stochasticity on droplet coarsening for asymptotically long times.

摘要

通过从固体基底上的薄流体膜去湿而自发形成液滴,可实现材料的纳米结构化。通常,能够控制液滴的演变并产生具有规则间隔液滴特征的图案至关重要。虽然热涨落在去湿过程中预计会发挥作用,但其相关性仍未得到很好的理解,尤其是在涉及液滴形成的非线性演变阶段。在随机润滑框架内,我们表明热噪声会显著影响液滴的形成过程。与确定性系统相比,随机系统的液滴数量较少,尺寸和空间分布的变化性更大。最后,我们讨论了渐近长时间下随机性对液滴粗化的影响。

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