Spectrum-dose conversion operator of NaI(Tl) and CsI(Tl) scintillation detectors for air dose rate measurement in contaminated environments.

Spectrum-dose conversion operators, the G(E) functions, for common NaI(Tl) scintillation survey meters and CsI(Tl) detectors are obtained for measurements in a semi-infinite plane of contaminated ground field by photon-emitting radionuclides (ground source). The calculated doses at a height of 100 cm from the ground in Cs-contaminated environments by the Monte Carlo simulation technique are compared with those obtained using the G(E) functions by assuming idealized irradiation geometries such as anterior-posterior or isotropic. The simulation reveals that one could overestimate air dose rates in the environment by a maximum of 20-30% for NaI(Tl) detectors and 40-50% for CsI(Tl) detectors depending on photon energy when using the G(E) functions assuming idealized irradiation geometries for ground source measurements. Measurements obtained after the nuclear accident in Fukushima reveal that the doses calculated using a G(E) function for a unidirectional irradiation geometry are 1.17 times higher than those calculated using a G(E) function for the ground source in the case of a CsI(Tl) scintillation detector, which has a rectangular parallelepiped crystal (13 × 13 × 20 mm). However, if a G(E) function is used assuming irradiation to a surface of the detector, the doses agree with those of the ground source within 2%. These results indicate that in contaminated environments, the commonly used scintillation-based detectors overestimate doses within the acceptable limit. In addition, the degree of overestimation depends on the irradiation direction of each detector assumed for developing the G(E) function. With regard to directional dependence of the detectors, reliable air dose rates in the environment can be obtained using the G(E) function determined in unidirectional irradiation geometry, provided that the irradiation surface of the crystal is determined properly.