Özgeriş Bünyamin, Göksu Süleyman, Polat Köse Leyla, Gülçin İlhami, Salmas Ramin Ekhteiari, Durdagi Serdar, Tümer Ferhan, Supuran Claudiu T
Erzurum Technical University, Faculty of Science, Department of Basic Sciences, Erzurum, Turkey; Ataturk University, Faculty of Science, Department of Chemistry, Erzurum, Turkey.
Ataturk University, Faculty of Science, Department of Chemistry, Erzurum, Turkey.
Bioorg Med Chem. 2016 May 15;24(10):2318-29. doi: 10.1016/j.bmc.2016.04.002. Epub 2016 Apr 2.
In the present study a series of urea and sulfamide compounds incorporating the tetralin scaffolds were synthesized and evaluated for their acetylcholinesterase (AChE), human carbonic anhydrase (CA, EC 4.2.1.1) isoenzyme I, and II (hCA I and hCA II) inhibitory properties. The urea and their sulfamide analogs were synthesized from the reactions of 2-aminotetralins with N,N-dimethylcarbamoyl chloride and N,N-dimethylsulfamoyl chloride, followed by conversion to the corresponding phenols via O-demethylation with BBr3. The novel urea and sulfamide derivatives were tested for inhibition of hCA I, II and AChE enzymes. These derivatives exhibited excellent inhibitory effects, in the low nanomolar range, with Ki values of 2.61-3.69nM against hCA I, 1.64-2.80nM against hCA II, and in the range of 0.45-1.74nM against AChE. In silico techniques such as, atomistic molecular dynamics (MD) and molecular docking simulations, were used to understand the scenario of the inhibition mechanism upon approaching of the ligands into the active site of the target enzymes. In light of the experimental and computational results, crucial amino acids playing a role in the stabilization of the enzyme-inhibitor adducts were identified.
在本研究中,合成了一系列含有四氢萘骨架的尿素和磺胺化合物,并对其乙酰胆碱酯酶(AChE)、人碳酸酐酶(CA,EC 4.2.1.1)同工酶I和II(hCA I和hCA II)的抑制特性进行了评估。尿素及其磺胺类似物由2-氨基四氢萘与N,N-二甲基甲酰氯和N,N-二甲基硫酰氯反应合成,然后用BBr₃进行O-去甲基化转化为相应的酚。测试了这些新型尿素和磺胺衍生物对hCA I、II和AChE酶的抑制作用。这些衍生物表现出优异的抑制效果,在低纳摩尔范围内,对hCA I的Ki值为2.61 - 3.69 nM,对hCA II的Ki值为1.64 - 2.80 nM,对AChE的Ki值在0.45 - 1.74 nM范围内。采用了诸如原子分子动力学(MD)和分子对接模拟等计算机模拟技术,以了解配体接近靶酶活性位点时的抑制机制情况。根据实验和计算结果,确定了在酶 - 抑制剂加合物稳定化过程中起作用的关键氨基酸。