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六角氮化硼中双曲声子极化激元反常内反射的成像。

Imaging of Anomalous Internal Reflections of Hyperbolic Phonon-Polaritons in Hexagonal Boron Nitride.

机构信息

U.S. Naval Research Laboratory , 4555 Overlook Avenue, S.W., Washington, DC 20375, United States.

Department of Physics, University of California San Diego , 9500 Gilman Drive, La Jolla, California 92093, United States.

出版信息

Nano Lett. 2016 Jun 8;16(6):3858-65. doi: 10.1021/acs.nanolett.6b01341. Epub 2016 May 13.

Abstract

We use scanning near-field optical microscopy to study the response of hexagonal boron nitride nanocones at infrared frequencies, where this material behaves as a hyperbolic medium. The obtained images are dominated by a series of "hot" rings that occur on the sloped sidewalls of the nanocones. The ring positions depend on the incident laser frequency and the nanocone shape. Both dependences are consistent with directional propagation of hyperbolic phonon-polariton rays that are launched at the edges and zigzag through the interior of the nanocones, sustaining multiple internal reflections off the sidewalls. Additionally, we observe a strong overall enhancement of the near-field signal at discrete resonance frequencies. These resonances attest to low dielectric losses that permit coherent standing waves of the subdiffractional polaritons to form. We comment on potential applications of such shape-dependent resonances and the field concentration at the hot rings.

摘要

我们使用扫描近场光学显微镜来研究在红外频率下六方氮化硼纳米锥的响应,在这个频率下,这种材料表现为双曲介质。所得到的图像主要由一系列“热点”环组成,这些环出现在纳米锥的斜侧壁上。环的位置取决于入射激光频率和纳米锥的形状。这两种依赖性都与双曲声子极化激元射线的定向传播一致,这些射线在边缘处发射,并在纳米锥内部曲折传播,在侧壁上多次反射。此外,我们还观察到在离散共振频率下近场信号的强烈整体增强。这些共振证明了低介电损耗的存在,允许亚衍射极化激元的相干驻波形成。我们评论了这种形状依赖性共振和热点环处的场集中的潜在应用。

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