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基态偶极²³Na⁸⁷Rb分子超冷气体的制备。

Creation of an Ultracold Gas of Ground-State Dipolar ^{23}Na^{87}Rb Molecules.

作者信息

Guo Mingyang, Zhu Bing, Lu Bo, Ye Xin, Wang Fudong, Vexiau Romain, Bouloufa-Maafa Nadia, Quéméner Goulven, Dulieu Olivier, Wang Dajun

机构信息

Department of Physics, The Chinese University of Hong Kong, Hong Kong, China.

Laboratoire Aimé Cotton, CNRS, Université Paris-Sud, ENS Cachan, Université Paris-Saclay, 91405 Orsay Cedex, France.

出版信息

Phys Rev Lett. 2016 May 20;116(20):205303. doi: 10.1103/PhysRevLett.116.205303. Epub 2016 May 19.

Abstract

We report the successful production of an ultracold sample of absolute ground-state ^{23}Na^{87}Rb molecules. Starting from weakly bound Feshbach molecules formed via magnetoassociation, the lowest rovibrational and hyperfine level of the electronic ground state is populated following a high-efficiency and high-resolution two-photon Raman process. The high-purity absolute ground-state samples have up to 8000 molecules and densities of over 10^{11}  cm^{-3}. By measuring the Stark shifts induced by external electric fields, we determined the permanent electric dipole moment of the absolute ground-state ^{23}Na^{87}Rb and demonstrated the capability of inducing an effective dipole moment over 1 D. Bimolecular reaction between ground-state ^{23}Na^{87}Rb molecules is endothermic, but we still observed a rather fast decay of the molecular sample. Our results pave the way toward investigation of ultracold molecular collisions in a fully controlled manner and possibly to quantum gases of ultracold bosonic molecules with strong dipolar interactions.

摘要

我们报告了成功制备出绝对基态(^{23}Na^{87}Rb)分子的超冷样本。从通过磁缔合形成的弱束缚费什巴赫分子开始,在高效高分辨率的双光子拉曼过程后,电子基态的最低振转和超精细能级被占据。高纯度的绝对基态样本包含多达8000个分子,密度超过(10^{11}\ cm^{-3})。通过测量外部电场引起的斯塔克位移,我们确定了绝对基态(^{23}Na^{87}Rb)的永久电偶极矩,并证明了诱导有效偶极矩超过1 D的能力。基态(^{23}Na^{87}Rb)分子之间的双分子反应是吸热的,但我们仍然观察到分子样本有相当快的衰变。我们的结果为以完全可控的方式研究超冷分子碰撞以及可能实现具有强偶极相互作用的超冷玻色子分子量子气体铺平了道路。

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