Wang Li-peng, Ma Yan, Zheng Jun, Cui Fen-ping, Zhou Yao-yao
Huan Jing Ke Xue. 2016 Mar 15;37(3):816-24.
In January 2013 large-scale, continuous and severe haze occurred in Nanjing. Three-wavelength photoacoustic soot spectrometer (PASS-3) was used for real-time, online and situ measurements of aerosol absorption and scattering coefficients in the northern suburb of Nanjing during January 2013. The results indicated that the average aerosol absorption and scattering coefficients were (83.20 ± 35.24) Mm⁻¹ and (670.16 ± 136.44) Mm⁻¹ during haze days, which were 3.85 and 3.45 times higher than those on clean days, respectively. The diurnal variation of absorption and scattering coefficients showed a bimodal distribution. The mean single scattering albedo and scattering Angstrom exponent were (0.89 ± 0.04) and (1.30 ± 0.27) respectively, indicating the predominance of scattering fine particles during haze days in Nanjing. Aerosols could be significantly removed by precipitation. The absorption and scattering coefficients showed negative correlations with surface wind speed, and the single scattering albedo and Angstrom exponent showed positive correlations with wind speed. Aerosol scattering coefficient was highest under southeasterly wind, whereas the absorption coefficient was highest under the southwesterly wind. In the three haze pollution events, Haze 1 and Haze 2 were mainly affected by long-range transportation of pollutants. Haze 1 was mainly affected by aging air mass from north Nanjing, Haze 2 was mainly affected by biomass burning air mass from southwest Nanjing, while Haze 3 was mainly caused by the high sulfate.
2013年1月,南京出现了大规模、持续且严重的雾霾天气。利用三波长光声烟尘光谱仪(PASS - 3)于2013年1月对南京北郊的气溶胶吸收系数和散射系数进行了实时、在线和原位测量。结果表明,雾霾天期间气溶胶平均吸收系数和散射系数分别为(83.20±35.24)Mm⁻¹和(670.16±136.44)Mm⁻¹,分别是清洁天的3.85倍和3.45倍。吸收系数和散射系数的日变化呈双峰分布。平均单次散射反照率和散射埃斯特朗指数分别为(0.89±0.04)和(1.30±0.27),表明南京雾霾天期间细颗粒物以散射为主。降水可显著去除气溶胶。吸收系数和散射系数与地面风速呈负相关,单次散射反照率和埃斯特朗指数与风速呈正相关。气溶胶散射系数在东南风条件下最高,而吸收系数在西南风条件下最高。在三次雾霾污染事件中,雾霾1和雾霾2主要受污染物远距离传输影响。雾霾1主要受南京北部老化气团影响,雾霾2主要受南京西南部生物质燃烧气团影响,而雾霾3主要由高硫酸盐所致。