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稠密玻璃态体系中的活性流化。

Active fluidization in dense glassy systems.

机构信息

Centre for Condensed Matter Theory, Department of Physics, Indian Institute of Science, Bangalore 560012, India.

Raman Research Institute, Bangalore 560080, India and National Centre for Biological Sciences (TIFR), Bangalore 560065, India.

出版信息

Soft Matter. 2016 Jul 20;12(29):6268-76. doi: 10.1039/c5sm02950c.

Abstract

Dense soft glasses show strong collective caging behavior at sufficiently low temperatures. Using molecular dynamics simulations of a model glass former, we show that the incorporation of activity or self-propulsion, f0, can induce cage breaking and fluidization, resulting in the disappearance of the glassy phase beyond a critical f0. The diffusion coefficient crosses over from being strongly to weakly temperature dependent as f0 is increased. In addition, we demonstrate that activity induces a crossover from a fragile to a strong glass and a tendency of active particles to cluster. Our results are of direct relevance to the collective dynamics of dense active colloidal glasses and to recent experiments on tagged particle diffusion in living cells.

摘要

密集软玻璃在足够低的温度下表现出强烈的集体笼状行为。使用模型玻璃形成体的分子动力学模拟,我们表明,活性或自推进的掺入,f0,可以诱导笼状破坏和流化,从而导致玻璃相在临界 f0 之外消失。当 f0 增加时,扩散系数从强烈依赖温度变为弱依赖温度。此外,我们证明活性诱导从易碎到强玻璃的转变以及活性粒子聚集的趋势。我们的结果与密集活性胶体玻璃的集体动力学以及最近在活细胞中标记粒子扩散的实验直接相关。

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