Liu Haoran, Liu Cheng, Xie Zhouqing, Li Ying, Huang Xin, Wang Shanshan, Xu Jin, Xie Pinhua
School of Earth and Space Sciences, University of Science and Technology of China, Hefei, 230026, China.
Key Lab of Environmental Optics &Technology, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China.
Sci Rep. 2016 Sep 29;6:34408. doi: 10.1038/srep34408.
A series of strict emission control measures were implemented in Beijing and surrounding regions to ensure good air quality during the 2014 Asia-Pacific Economic Cooperation (APEC) summit and 2015 Grand Military Parade (Parade), which led to blue sky days during these two events commonly referred to as "APEC Blue" and "Parade Blue". Here we calculated Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) and Ozone Monitoring Instrument (OMI) NO and HCHO results based on well known DOAS trace gas fitting algorithm and WRF-Chem model (with measured climatology parameter and newest emission inventor) simulated trace gases profiles. We found the NO columns abruptly decreased both Parade (43%) and APEC (21%) compared with the periods before these two events. The back-trajectory cluster analysis and the potential source contribution function (PSCF) proved regional transport from southern peripheral cities plays a key role in pollutants observed at Beijing. The diminishing transport contribution from southern air mass during Parade manifests the real effect of emission control measures on NO pollution. Based on the ratios of HCHO over NO we found there were not only limited the NO pollutant but also suppress the O contaminant during Parade, while O increased during the APEC.
北京及周边地区实施了一系列严格的排放控制措施,以确保2014年亚太经合组织(APEC)峰会和2015年大阅兵期间的空气质量良好,这使得这两个活动期间出现了蓝天,通常被称为“APEC蓝”和“阅兵蓝”。在此,我们基于著名的差分光学吸收光谱法(DOAS)痕量气体拟合算法和WRF-Chem模型(使用实测气候学参数和最新排放清单)模拟的痕量气体剖面,计算了多轴差分光学吸收光谱仪(MAX-DOAS)和臭氧监测仪(OMI)的NO和HCHO结果。我们发现,与这两个活动之前的时期相比,阅兵期间(43%)和APEC期间(21%)的NO柱均急剧下降。后向轨迹聚类分析和潜在源贡献函数(PSCF)证明,来自南部周边城市的区域传输在北京观测到的污染物中起关键作用。阅兵期间来自南部气团的传输贡献减少,体现了排放控制措施对NO污染的实际影响。基于HCHO与NO的比值,我们发现阅兵期间不仅限制了NO污染物,还抑制了O污染物,而APEC期间O有所增加。