Yu Fan, Hirschberger Max, Loew Toshinao, Li Gang, Lawson Benjamin J, Asaba Tomoya, Kemper J B, Liang Tian, Porras Juan, Boebinger Gregory S, Singleton John, Keimer Bernhard, Li Lu, Ong N Phuan
Department of Physics, University of Michigan, Ann Arbor, MI 48109.
Department of Physics, Princeton University, Princeton, NJ 08544.
Proc Natl Acad Sci U S A. 2016 Nov 8;113(45):12667-12672. doi: 10.1073/pnas.1612591113. Epub 2016 Oct 24.
Strong evidence for charge-density correlation in the underdoped phase of the cuprate YBaCuO was obtained by NMR and resonant X-ray scattering. The fluctuations were found to be enhanced in strong magnetic fields. Recently, 3D charge-density-wave (CDW) formation with long-range order (LRO) was observed by X-ray diffraction in [Formula: see text] 15 T. To elucidate how the CDW transition impacts the pair condensate, we have used torque magnetization to 45 T and thermal conductivity [Formula: see text] to construct the magnetic phase diagram in untwinned crystals with hole density = 0.11. We show that the 3D CDW transitions appear as sharp features in the susceptibility and [Formula: see text] at the fields [Formula: see text] and [Formula: see text], which define phase boundaries in agreement with spectroscopic techniques. From measurements of the melting field [Formula: see text] of the vortex solid, we obtain evidence for two vortex solid states below 8 K. At 0.5 K, the pair condensate appears to adjust to the 3D CDW by a sharp transition at 24 T between two vortex solids with very different shear moduli. At even higher (41 T), the second vortex solid melts to a vortex liquid which survives to fields well above 41 T. de Haas-van Alphen oscillations appear at fields 24-28 T, below the lower bound for the upper critical field [Formula: see text].
通过核磁共振(NMR)和共振X射线散射,在铜酸盐YBaCuO的欠掺杂相中获得了电荷密度相关性的有力证据。发现这些涨落在强磁场中增强。最近,通过X射线衍射在15 T下观察到具有长程序(LRO)的三维电荷密度波(CDW)形成。为了阐明CDW转变如何影响配对凝聚,我们使用扭矩磁化到45 T和热导率来构建空穴密度为0.11的非孪晶晶体中的磁相图。我们表明,三维CDW转变在磁化率和热导率中表现为在磁场[公式:见正文]和[公式:见正文]处的尖锐特征,这些磁场定义了与光谱技术一致的相界。通过对涡旋固体的熔化场[公式:见正文]的测量,我们获得了低于8 K的两种涡旋固体状态的证据。在0.5 K时,配对凝聚似乎通过在24 T处的尖锐转变,在具有非常不同剪切模量的两种涡旋固体之间适应三维CDW。在更高的磁场(41 T)下,第二种涡旋固体熔化为一种涡旋液体,该液体在远高于41 T的磁场中仍然存在。德哈斯 - 范阿尔芬振荡出现在24 - 28 T的磁场中,低于上临界场[公式:见正文]的下限。