Leroux Maxime, Mishra Vivek, Ruff Jacob P C, Claus Helmut, Smylie Matthew P, Opagiste Christine, Rodière Pierre, Kayani Asghar, Gu G D, Tranquada John M, Kwok Wai-Kwong, Islam Zahirul, Welp Ulrich
Materials Science Division, Argonne National Laboratory, Lemont, IL 60439;
Materials Science Division, Argonne National Laboratory, Lemont, IL 60439.
Proc Natl Acad Sci U S A. 2019 May 28;116(22):10691-10697. doi: 10.1073/pnas.1817134116. Epub 2019 May 13.
With the discovery of charge-density waves (CDWs) in most members of the cuprate high-temperature superconductors, the interplay between superconductivity and CDWs has become a key point in the debate on the origin of high-temperature superconductivity. Some experiments in cuprates point toward a CDW state competing with superconductivity, but others raise the possibility of a CDW-superconductivity intertwined order or more elusive pair-density waves (PDWs). Here, we have used proton irradiation to induce disorder in crystals of [Formula: see text] and observed a striking 50% increase of [Formula: see text], accompanied by a suppression of the CDWs. This is in sharp contrast with the behavior expected of a d-wave superconductor, for which both magnetic and nonmagnetic defects should suppress [Formula: see text] Our results thus make an unambiguous case for the strong detrimental effect of the CDW on bulk superconductivity in [Formula: see text] Using tunnel diode oscillator (TDO) measurements, we find indications for potential dynamic layer decoupling in a PDW phase. Our results establish irradiation-induced disorder as a particularly relevant tuning parameter for the many families of superconductors with coexisting density waves, which we demonstrate on superconductors such as the dichalcogenides and [Formula: see text].
随着在大多数铜酸盐高温超导体中发现电荷密度波(CDW),超导性与CDW之间的相互作用已成为高温超导起源辩论中的一个关键点。铜酸盐中的一些实验表明CDW态与超导性相互竞争,但其他实验则提出了CDW - 超导性交织序或更难以捉摸的对密度波(PDW)的可能性。在这里,我们使用质子辐照在[化学式:见原文]晶体中引入无序,并观察到[化学式:见原文]显著增加了50%,同时伴随着CDW的抑制。这与d波超导体预期的行为形成鲜明对比,对于d波超导体,磁性和非磁性缺陷都应抑制[化学式:见原文]。因此,我们的结果明确证明了CDW对[化学式:见原文]体超导性有强烈的不利影响。使用隧道二极管振荡器(TDO)测量,我们发现了在PDW相中潜在动态层解耦的迹象。我们的结果表明,辐照诱导的无序是许多共存密度波的超导体系特别相关的调节参数,我们在二硫属化物和[化学式:见原文]等超导体上证明了这一点。