Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou 510006, China.
Nanoscale. 2016 Dec 7;8(45):18963-18971. doi: 10.1039/c6nr06504j. Epub 2016 Nov 3.
The interaction of silicon (Si) nanospheres (NSs) with a thin metal film is investigated numerically and experimentally by characterizing their forward scattering properties. A sharp resonant mode and a zero-scattering dip are found to be introduced in the forward scattering spectrum of a Si NS by putting it on a 50-nm-thick gold film. It is revealed that the sharp resonant mode arises from a new magnetic dipole induced by the electric dipole and its mirror image while the zero-scattering dip originates from the destructive interference between the new magnetic dipole and the original one together with its mirror image. A significant enhancement in both electric and magnetic fields is achieved at the contact point between the Si NS and the metal film. More interestingly, the use of a thin silver film can lead to vivid scattering light with different color indices. It is demonstrated that a small change in the surrounding environment of Si NSs results in the broadening of the resonant mode and the disappearance of the zero-scattering dip. Our findings indicate that dielectric-metal hybrid systems composed of semiconductor NSs and thin metal films act as attractive platforms on which novel nanoscale plasmonic devices can be realized.
通过对其前向散射特性的表征,数值和实验研究了硅纳米球(NSs)与薄金属膜的相互作用。研究发现,将硅 NS 置于 50nm 厚的金膜上会在其前向散射光谱中引入尖锐的共振模式和零散射陷波。结果表明,尖锐的共振模式源于电偶极子及其镜像诱导的新磁偶极子,而零散射陷波则源于新磁偶极子与原始磁偶极子及其镜像之间的相消干涉。在硅 NS 与金属膜的接触点处实现了电场和磁场的显著增强。更有趣的是,使用薄银膜可以产生具有不同颜色指数的生动散射光。结果表明,硅 NS 周围环境的微小变化会导致共振模式变宽和零散射陷波消失。我们的研究结果表明,由半导体 NS 和薄金属膜组成的介电-金属混合系统是实现新型纳米级等离子体器件的有吸引力的平台。