Lever Michael, McEntyre Christopher J, George Peter M, Chambers Stephen T
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Biol Chem. 2017 Jun 27;398(7):775-784. doi: 10.1515/hsz-2016-0261.
Choline metabolism is by oxidation to betaine, which is demethylated to N,N-dimethylglycine; dimethylglycine is oxidatively demethylated to sarcosine. This pathway is important for osmoregulation and as a source of methyl groups. We asked whether another metabolite was involved. We synthesized the N-oxide of dimethylglycine (DMGO) by oxidizing dimethylglycine with peracetic acid, and measured DMGO in human plasma and urine by HPLC-MS/MS with positive ion detection, using two chromatography procedures, based on ion exchange and HILIC separations. The molecular ion DMGOH+ (m/z=120) yielded four significant fragments (m/z=103, 102, 58 and 42). The suspected DMGO peak in human body fluids showed all these fragments, and co-chromatographed with added standard DMGO in both HPLC systems. Typical plasma concentrations of DMGO are under 1 μmol/l. They may be lower in metabolic syndrome patients. Urine concentrations are higher, and DMGO has a higher fractional clearance than dimethylglycine, betaine and choline. It was present in all of over 80 human urine and plasma samples assayed. Plasma DMGO concentrations correlate with plasma DMG concentrations, with betaine and choline concentrations, with the osmolyte myo-inositol, and strongly with urinary DMGO excretion. We conclude that DMGO is probably a normal human metabolite.
胆碱代谢是通过氧化生成甜菜碱,甜菜碱再脱甲基生成N,N-二甲基甘氨酸;二甲基甘氨酸经氧化脱甲基生成肌氨酸。这条途径对于渗透调节以及作为甲基来源都很重要。我们研究是否有另一种代谢产物参与其中。我们用过氧乙酸氧化二甲基甘氨酸合成了二甲基甘氨酸N-氧化物(DMGO),并使用基于离子交换和亲水相互作用液相色谱分离的两种色谱方法,通过高效液相色谱-串联质谱法(HPLC-MS/MS)在正离子检测模式下测定人血浆和尿液中的DMGO。分子离子DMGOH⁺(m/z = 120)产生了四个显著的碎片(m/z = 103、102、58和42)。人体体液中疑似DMGO的峰显示出所有这些碎片,并且在两个HPLC系统中都与添加的标准DMGO共色谱。DMGO的典型血浆浓度低于1μmol/L。代谢综合征患者的浓度可能更低。尿液浓度更高,并且DMGO的分数清除率高于二甲基甘氨酸、甜菜碱和胆碱。在所有检测的80多个尿液和血浆样本中均有发现。血浆DMGO浓度与血浆二甲基甘氨酸浓度、甜菜碱和胆碱浓度、渗透压溶质肌醇相关,并且与尿DMGO排泄密切相关。我们得出结论,DMGO可能是一种正常的人体代谢产物。