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二硫化铼的非线性饱和和偏振诱导吸收。

Nonlinear Saturable and Polarization-induced Absorption of Rhenium Disulfide.

机构信息

State Key Laboratory of Modern Optical Instrumentation, Department of Optical Engineering, Zhejiang University, Hangzhou 310027, China.

State Key Laboratory of Transient Optics and Photonics, Xi'an Institute of Optics and Precision Mechanics, Chinese Academy of Sciences, Xi'an 710119, China.

出版信息

Sci Rep. 2017 Jan 5;7:40080. doi: 10.1038/srep40080.

DOI:10.1038/srep40080
PMID:28053313
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5215599/
Abstract

Monolayer of transition metal dichalcogenides (TMDs), with lamellar structure as that of graphene, has attracted significant attentions in optoelectronics and photonics. Here, we focus on the optical absorption response of a new member TMDs, rhenium disulphide (ReS) whose monolayer and bulk forms have the nearly identical band structures. The nonlinear saturable and polarization-induced absorption of ReS are investigated at near-infrared communication band beyond its bandgap. It is found that the ReS-covered D-shaped fiber (RDF) displays the remarkable polarization-induced absorption, which indicates the different responses for transverse electric (TE) and transverse magnetic (TM) polarizations relative to ReS plane. Nonlinear saturable absorption of RDF exhibits the similar saturable fluence of several tens of μJ/cm and modulation depth of about 1% for ultrafast pulses with two orthogonal polarizations. RDF is utilized as a saturable absorber to achieve self-started mode-locking operation in an Er-doped fiber laser. The results broaden the operation wavelength of ReS from visible light to around 1550 nm, and numerous applications may benefit from the anisotropic and nonlinear absorption characteristics of ReS, such as in-line optical polarizers, high-power pulsed lasers, and optical communication system.

摘要

过渡金属二硫属化物(TMDs)的单层结构,具有类似于石墨烯的层状结构,在光电子学和光子学领域引起了广泛关注。在这里,我们专注于 TMDs 的一个新成员——二硫化铼(ReS)的光学吸收响应,其单层和体相具有几乎相同的能带结构。我们在近红外通讯波段(超过其带隙)研究了 ReS 的非线性饱和和偏振诱导吸收。结果发现,ReS 覆盖的 D 形光纤(RDF)表现出显著的偏振诱导吸收,这表明相对于 ReS 平面,其对横电(TE)和横磁(TM)偏振有不同的响应。RDF 的非线性饱和吸收表现出类似的饱和光强,对于两个正交偏振的超快脉冲,其饱和光强约为几十微焦耳每平方厘米,调制深度约为 1%。RDF 被用作可饱和吸收体,在掺铒光纤激光器中实现了自启动的锁模运转。这些结果将 ReS 的工作波长从可见光扩展到约 1550nm,并且 ReS 的各向异性和非线性吸收特性可能会在许多应用中受益,例如在线光学偏振器、高功率脉冲激光器和光通信系统。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/143747b2e673/srep40080-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/cd481cb9ed6f/srep40080-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/593f7585d921/srep40080-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/dfb5f7e5400b/srep40080-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/283735b36635/srep40080-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/2e6cc84a8f92/srep40080-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/143747b2e673/srep40080-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/cd481cb9ed6f/srep40080-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/593f7585d921/srep40080-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/dfb5f7e5400b/srep40080-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/283735b36635/srep40080-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/2e6cc84a8f92/srep40080-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/91f8/5215599/143747b2e673/srep40080-f6.jpg

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本文引用的文献

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