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混合石墨烯/氮化硼纳米带中的温控巨磁电阻和完美自旋塞贝克效应。

Temperature-controlled colossal magnetoresistance and perfect spin Seebeck effect in hybrid graphene/boron nitride nanoribbons.

作者信息

Zhu Lin, Li Ruimin, Yao Kailun

机构信息

School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074, China.

出版信息

Phys Chem Chem Phys. 2017 Feb 1;19(5):4085-4092. doi: 10.1039/c6cp07179a.

Abstract

Thermal spin transport properties of graphene and hexagonal boron nitride nanoribbon heterojunctions have been investigated using density functional theory calculations combined with the Keldysh nonequilibrium Green's function approach. The results showed that the perfect spin Seebeck effect and analogy negative differential thermoelectric resistance occurred in the device under a temperature difference without a gate or bias voltage. An intriguing thermally induced colossal magnetoresistance without gate regulation was also observed, which can be switched between a positive and negative value with temperature control. It was also found that the unit number of zigzag graphene nanoribbons and boron nitride nanoribbons can tune the electronic band structure and the energy gap of the heterostructure, and then modulate the thermal spin transport properties. The results suggest that graphene and hexagonal boron nitride nanoribbon heterostructures may have potential applications in graphene-based nanodevices.

摘要

利用密度泛函理论计算结合凯尔迪什非平衡格林函数方法,研究了石墨烯与六方氮化硼纳米带异质结的热自旋输运性质。结果表明,在无栅极或偏置电压的温差条件下,该器件中出现了完美的自旋塞贝克效应和类似的负微分热电阻。还观察到一种有趣的无栅极调控的热致巨磁电阻,其可通过温度控制在正值和负值之间切换。还发现锯齿形石墨烯纳米带和氮化硼纳米带的单元数量可以调节异质结构的电子能带结构和能隙,进而调制热自旋输运性质。结果表明,石墨烯与六方氮化硼纳米带异质结构在基于石墨烯的纳米器件中可能具有潜在应用。

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