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颗粒棒振动单层中的凝聚。

Clustering in vibrated monolayers of granular rods.

机构信息

Departamento de Física Teórica de la Materia Condensada, Universidad Autónoma de Madrid, E-28049, Madrid, Spain.

Departamento de Química, Universidad Autónoma de Madrid, E-28049, Madrid, Spain.

出版信息

Soft Matter. 2017 Apr 5;13(14):2571-2582. doi: 10.1039/c7sm00102a.

Abstract

We investigate the ordering properties of vertically-vibrated monolayers of granular cylinders in a circular container at high packing fraction. In line with previous works by other groups, we identify liquid-crystalline ordering behaviour similar to that of two-dimensional hard rectangular particles subject to thermal equilibrium fluctuations. However, due to dissipation, there is a much stronger tendency for particles to cluster into parallel arrangements in the granular system. These clusters behave as a polydisperse mixture of long life-time 'superparticles', and some aspects of the system behaviour can be understood by applying mean-field theories for equilibrium hard rectangles, based on two-body correlations, to these 'superparticles'. Many other features of the granular system are different: (i) for small particle length-to-breadth ratio κ, we identify tetratic ordering at moderate packing fractions and smectic fluctuations at higher packing fractions, with no sharp transition between the two states. Both types of ordering can be explained in terms of clustering. (ii) For large κ, strong clustering precludes the stabilisation of a uniaxial nematic state, and the system exhibits a mixture of randomly-oriented clusters which, as packing fraction is increased, develops into states with smectic fluctuations, again through a diffuse transition. (iii) Vorticity excitations of the velocity field compete with smectic ordering, causing dynamic fluctuations and the absence of steady states at high densities; the tetratic state, by contrast, is very stiff against vorticity, and long-standing steady states, spatially and orientationally homogeneous except for four symmetrical defects located close to the wall, can be observed.

摘要

我们研究了在高填充率下,圆形容器中垂直振动的颗粒圆柱体单层的有序性质。与其他小组的先前工作一致,我们确定了类似于二维硬矩形颗粒在热平衡波动下的液晶有序行为。然而,由于耗散,颗粒在颗粒系统中更强烈地倾向于聚类成平行排列。这些聚类表现为长寿命“超粒子”的多分散混合物,并且可以通过将基于二体相关的平衡硬矩形的平均场理论应用于这些“超粒子”来理解系统行为的某些方面。颗粒系统的许多其他特征不同:(i)对于小的颗粒长径比 κ,我们在中等填充率下确定了四方有序,在较高填充率下确定了近晶波动,两种状态之间没有明显的转变。这两种类型的有序都可以通过聚类来解释。(ii)对于大的 κ,强烈的聚类阻止了单轴向列状态的稳定,系统表现出随机取向的聚类混合物,随着填充率的增加,通过弥散转变发展为具有近晶波动的状态。(iii)速度场的涡度激发与近晶有序竞争,导致高密度下的动态波动和稳态的缺失;相比之下,四方态对涡度非常僵硬,可以观察到除了靠近壁的四个对称缺陷外,空间和取向均匀的长时间稳态。

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