Liu Yang, Vashishta Manish, Djuricanin Pavle, Zhou Sida, Zhong Wei, Mittertreiner Tony, Carty David, Momose Takamasa
Department of Chemistry, The University of British Columbia, Vancouver, British Columbia V6T 1Z1, Canada.
Department of Physics and Astronomy, The University of British Columbia, Vancouver, British Columbia V6T 1Z1, Canada.
Phys Rev Lett. 2017 Mar 3;118(9):093201. doi: 10.1103/PhysRevLett.118.093201. Epub 2017 Feb 27.
We have demonstrated that a supersonic beam of methyl radicals (CH_{3}) in the ground rotational state of both para and ortho species has been slowed down to standstill with a magnetic molecular decelerator, and successfully captured spatially in an anti-Helmholtz magnetic trap for >1 s. The trapped CH_{3} radicals have a mean translational temperature of about 200 mK with an estimated density of >5.0×10^{7} cm^{-3}. The methyl radical is an ideal system for the study of cold molecules not only because of its high reactivities at low temperatures, but also because further cooling below 1 mK is plausible via sympathetic cooling with ultracold atoms. The demonstrated trapping capability of methyl radicals opens up various possibilities for realizing ultracold ensembles of molecules towards Bose-Einstein condensation of polyatomic molecules and investigations of reactions governed by quantum statistics.
我们已经证明,处于仲氢和正氢物种基态旋转状态的超音速甲基自由基(CH₃)束已被磁分子减速器减速至静止,并成功地在反亥姆霍兹磁阱中被空间捕获超过1秒。被捕获的CH₃自由基的平均平移温度约为200 mK,估计密度大于5.0×10⁷ cm⁻³。甲基自由基是研究冷分子的理想系统,不仅因为它在低温下具有高反应活性,还因为通过与超冷原子的交感冷却,进一步冷却至低于1 mK是可行的。所展示的甲基自由基捕获能力为实现分子的超冷系综以实现多原子分子的玻色-爱因斯坦凝聚以及研究由量子统计支配的反应开辟了各种可能性。