Liquid Crystal Institute and Chemical Physics Interdisciplinary Program, Kent State University, Kent, Ohio 44242, USA.
Nat Commun. 2017 Apr 21;8:14974. doi: 10.1038/ncomms14974.
The detailed structure of singularities of ordered field represents a fundamental problem in diverse areas of physics. At the defect cores, the deformations are so strong that the system explores states with symmetry different from that of an undistorted material. These regions are difficult to explore experimentally as their spatial extension is very small, a few molecular lengths in the condensed matter. Here we explore the cores of disclinations in the so-called chromonic nematics that extend over macroscopic length scales accessible for optical characterization. We demonstrate that the amplitude S and the phase (the director) of the order parameter vary along both the radial and azimuthal directions, in contrast to the classic models in which S varies only with the distance from the centre and depends only on the azimuthal coordinate. This unexpected core structure is explained by a strong coupling of the phase and amplitude of the order parameter in the free energy.
有序场奇点的详细结构代表了物理学不同领域的一个基本问题。在缺陷核心处,变形非常强烈,以至于系统探索的状态具有与未失真材料不同的对称性。由于这些区域的空间延伸非常小,只有凝聚态物质中的几个分子长度,因此很难通过实验进行探索。在这里,我们研究了所谓的手性向列液晶中螺旋位错的核心,这些核心延伸到可用于光学表征的宏观长度尺度。我们证明,有序参数的幅度 S 和相位(指向矢)沿径向和角向两个方向变化,这与经典模型不同,经典模型中 S 仅随离中心的距离而变化,并且仅取决于角坐标。这种意想不到的核心结构可以通过自由能中有序参数的相位和幅度的强耦合来解释。