Harkai Saša, Murray Bryce S, Rosenblatt Charles, Kralj Samo
Condensed Matter Physics, Jožef Stefan Institute, SI-1000 Ljubljana, Slovenia.
Department of Physics, Case Western Reserve University Cleveland, Ohio 44106, USA.
Phys Rev Res. 2020 Feb;2(1). doi: 10.1103/physrevresearch.2.013176. Epub 2020 Feb 20.
Topological defects appear in symmetry breaking phase transitions and are ubiquitous throughout Nature. As an ideal testbed for their study, defect configurations in nematic liquid crystals (NLCs) could be exploited in a rich variety of technological applications. Here we report on robust theoretical and experimental investigations in which an external electric field is used to switch between pre-determined stable chargeless disclination patterns in a nematic cell, where the cell is sufficiently thick that the disclinations start and terminate at the same surface. The different defect configurations are stabilised by a master substrate that enforces a lattice of surface defects exhibiting zero total topological charge value. Theoretically, we model disclination configurations using a Landau-de Gennes phenomenological model. Experimentally, we enable diverse defect patterns by implementing an in-house-developed Atomic Force Measurement scribing method, where NLC configurations are monitored via polarised optical microscopy. We show numerically and experimentally that an "alphabet" of up to 18 unique line defect configurations can be stabilised in a 4x4 lattice of alternating s=±1 surface defects, which can be "rewired" multistably using appropriate field manipulation. Our proof-of-concept mechanism may lead to a variety of applications, such as multistable optical displays and rewirable nanowires. Our studies also are of interest from a fundamental perspective. We demonstrate that a chargeless line could simultaneously exhibit defect-antidefect properties. Consequently, a pair of such antiparallel disclinations exhibits an attractive interaction. For a sufficiently closely-spaced pair of substrate-pinned defects, this interaction could trigger rewiring, or annihilation if defects are depinned.
拓扑缺陷出现在对称破缺相变中,在自然界中无处不在。作为研究它们的理想试验台,向列型液晶(NLC)中的缺陷构型可用于各种各样的技术应用。在此,我们报告了深入的理论和实验研究,其中利用外部电场在向列型液晶盒中预先确定的稳定无电荷向错图案之间进行切换,该液晶盒足够厚,使得向错在同一表面开始和终止。不同的缺陷构型由一个主基板稳定,该主基板强制形成一个表面缺陷晶格,其总拓扑电荷值为零。从理论上讲,我们使用朗道 - 德热纳唯象模型对向错构型进行建模。在实验中,我们通过实施自行开发的原子力测量刻划方法实现了多种缺陷图案,其中通过偏振光学显微镜监测NLC构型。我们通过数值和实验表明,在交替的s = ±1表面缺陷的4x4晶格中,可以稳定多达18种独特线缺陷构型的“字母表”,可以使用适当的场操纵对其进行多稳态“重新布线”。我们的概念验证机制可能会带来各种应用,例如多稳态光学显示器和可重新布线的纳米线。从基础角度来看,我们的研究也很有意义。我们证明了无电荷线可以同时表现出缺陷 - 反缺陷特性。因此,一对这样的反平行向错表现出吸引相互作用。对于一对足够紧密间隔的由基板固定的缺陷,这种相互作用可能会触发重新布线,如果缺陷被解除固定则会导致湮灭。