Meteorological Institute, Ludwig-Maximilians-Universität München, Munich, Germany.
Sci Total Environ. 2017 Oct 15;596-597:212-221. doi: 10.1016/j.scitotenv.2017.04.091. Epub 2017 Apr 20.
In this paper, we present a quantitative estimation of the impacts of biomass burning emissions from different source regions to the local air quality in Hong Kong in 2014 using global chemistry transport model simulations, sun photometer measurements, satellite observations and local monitoring network data. This study focuses on two major biomass burning pollutants, black carbon aerosols and carbon monoxide (CO). The model simulations of atmospheric black carbon and CO show excellent agreement with sun photometer aerosol optical depth (AOD) measurements, satellite CO columns observations and local monitoring stations data. From the model simulation results, we estimated that biomass burning contributes 12% of total black carbon and 16% of atmospheric CO in Hong Kong on annual average. South East Asia shows the largest influence to the black carbon and CO levels in Hong Kong, accounts for 11% of the total atmospheric black carbon and 8% of CO. Biomass burning in North East Asia and Africa also show significant impacts to Hong Kong. Elevated levels of atmospheric black carbon aerosols and CO were observed during springtime (March and April) which is mainly due to the enhancement of biomass burning contributions. Black carbon and CO originating from biomass burning sources are estimated to contribute 40% of atmospheric black carbon and 28% of CO in Hong Kong during March 2014. An investigation focusing on the biomass burning pollution episode during springtime suggests the intensified biomass burning activities in the Indochinese Peninsula are the major sources of black carbon and CO in Hong Kong during the time.
本文利用全球化学输送模式模拟、太阳光度计测量、卫星观测和本地监测网络数据,定量评估了 2014 年不同源区生物质燃烧排放对香港本地空气质量的影响。本研究重点关注两种主要的生物质燃烧污染物,即黑碳气溶胶和一氧化碳(CO)。大气黑碳和 CO 的模式模拟与太阳光度计气溶胶光学深度(AOD)测量、卫星 CO 柱观测和本地监测站数据吻合良好。根据模型模拟结果,我们估计生物质燃烧对香港地区黑碳和 CO 的年均贡献分别为 12%和 16%。东南亚对香港的黑碳和 CO 水平影响最大,占大气黑碳总量的 11%和 CO 的 8%。东北亚和非洲的生物质燃烧也对香港有显著影响。在春季(三月和四月)观测到大气黑碳气溶胶和 CO 浓度升高,主要是由于生物质燃烧贡献的增强。在 2014 年 3 月,估计来自生物质燃烧源的黑碳和 CO 分别占香港大气黑碳和 CO 的 40%和 28%。对春季生物质燃烧污染事件的调查表明,此时越南半岛的生物质燃烧活动加剧是香港黑碳和 CO 的主要来源。