Universität Göttingen, Geowissenschaftliches Zentrum, Goldschmidtstraße 1, 37077 Göttingen, Germany.
Karlsruher Institut für Technologie, Institut für Angewandte Materialien - Werkstoffprozesstechnik, Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany.
Nat Commun. 2017 Jun 1;8:15702. doi: 10.1038/ncomms15702.
Molten I-type cosmic spherules formed by heating, oxidation and melting of extraterrestrial Fe,Ni metal alloys. The entire oxygen in these spherules sources from the atmosphere. Therefore, I-type cosmic spherules are suitable tracers for the isotopic composition of the upper atmosphere at altitudes between 80 and 115 km. Here we present data on I-type cosmic spherules collected in Antarctica. Their composition is compared with the composition of tropospheric O. Our data suggest that the Earth's atmospheric O is isotopically homogenous up to the thermosphere. This makes fossil I-type micrometeorites ideal proxies for ancient atmospheric CO levels.
熔融 I 型宇宙球粒是由外星 Fe、Ni 金属合金加热、氧化和熔化形成的。这些球粒中的全部氧都来源于大气。因此,I 型宇宙球粒是 80-115 公里高空上层大气同位素组成的合适示踪剂。本文给出了在南极洲采集的 I 型宇宙球粒的数据。将其组成与对流层 O 的组成进行了比较。我们的数据表明,地球大气中的 O 同位素在热层达到均一。这使得化石 I 型微陨石成为古代大气 CO 水平的理想示踪物。