Tuccitto Nunzio, Li-Destri Giovanni, Messina Grazia M L, Marletta Giovanni
Laboratory for Molecular Surfaces and Nanotechnology (LAMSUN), Department of Chemical Science, University of Catania and CSGI , viale A. Doria 6, 95125 Catania, Italy.
J Phys Chem Lett. 2017 Aug 17;8(16):3861-3866. doi: 10.1021/acs.jpclett.7b01713. Epub 2017 Aug 4.
The modeling and realization of an effective communication platform for long-range information transfer is reported. Messages are encrypted in molecular bits by concentration pulses of fluorescent carbon quantum dots having self-quenching emission that dynamically depends on the concentration pulses. Messages are transferred along longer paths when received and decoded by means of dynamical emission response with respect to the ones encoded by absorbance scaling linearly with messenger concentration. These results represent a significant breakthrough in view of the futuristic development of a nonspecific molecular communication platform to encode and transfer information in multiple fluid environments, ranging from physiological to industrial ones.
报道了一种用于远程信息传输的有效通信平台的建模与实现。通过具有自猝灭发射的荧光碳量子点的浓度脉冲将消息加密为分子比特,该自猝灭发射动态地取决于浓度脉冲。当通过动态发射响应接收和解码消息时,与通过信使浓度线性缩放吸光度编码的消息相比,消息能够沿着更长的路径进行传输。鉴于未来非特异性分子通信平台在多种流体环境(从生理环境到工业环境)中编码和传输信息的发展,这些结果代表了一项重大突破。