Paschen Timo, Förster Michael, Krüger Michael, Lemell Christoph, Wachter Georg, Libisch Florian, Madlener Thomas, Burgdörfer Joachim, Hommelhoff Peter
Department of Physics, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Erlangen, Germany.
Max Planck Institute of Quantum Optics, Garching, Germany.
J Mod Opt. 2017 Jun 17;64(10-11):1054-1060. doi: 10.1080/09500340.2017.1281453. Epub 2017 Jan 29.
In this article, we present coherent control of above-threshold photoemission from a tungsten nanotip achieving nearly perfect modulation. Depending on the pulse delay between fundamental ([Formula: see text]) and second harmonic ([Formula: see text]) pulses of a femtosecond fiber laser at the nanotip, electron emission is significantly enhanced or depressed during temporal overlap. Electron emission is studied as a function of pulse delay, optical near-field intensities, DC bias field and final photoelectron energy. Under optimized conditions modulation amplitudes of the electron emission of 97.5% are achieved. Experimental observations are discussed in the framework of quantum-pathway interference supported by local density of states simulations.
在本文中,我们展示了对钨纳米尖端阈上光发射的相干控制,实现了近乎完美的调制。根据飞秒光纤激光器在纳米尖端的基频([公式:见原文])和二次谐波([公式:见原文])脉冲之间的脉冲延迟,在时间重叠期间电子发射会显著增强或抑制。研究了电子发射与脉冲延迟、光学近场强度、直流偏置场和最终光电子能量的函数关系。在优化条件下,实现了97.5%的电子发射调制幅度。在由局域态密度模拟支持的量子路径干涉框架内讨论了实验观察结果。