Haas Derek A, Eslinger Paul W, Bowyer Theodore W, Cameron Ian M, Hayes James C, Lowrey Justin D, Miley Harry S
Pacific Northwest National Laboratory, 902 Battelle Blvd., Richland, WA, 99354, USA; The University of Texas at Austin, 110 Inner Campus Drive, Austin, TX, 78712, USA.
Pacific Northwest National Laboratory, 902 Battelle Blvd., Richland, WA, 99354, USA.
J Environ Radioact. 2017 Nov;178-179:127-135. doi: 10.1016/j.jenvrad.2017.08.005. Epub 2017 Aug 14.
The Comprehensive Nuclear-Test-Ban Treaty bans all nuclear tests and mandates development of verification measures to detect treaty violations. One verification measure is detection of radioactive xenon isotopes produced in the fission of actinides. The International Monitoring System (IMS) currently deploys automated radioxenon systems that can detect four radioxenon isotopes. Radioxenon systems with lower detection limits are currently in development. Historically, the sensitivity of radioxenon systems was measured by the minimum detectable concentration for each isotope. In this paper we analyze the response of radioxenon systems using rigorous metrics in conjunction with hypothetical representative releases indicative of an underground nuclear explosion instead of using only minimum detectable concentrations. Our analyses incorporate the impact of potential spectral interferences on detection limits and the importance of measuring isotopic ratios of the relevant radioxenon isotopes in order to improve discrimination from background sources particularly for low-level releases. To provide a sufficient data set for analysis, hypothetical representative releases are simulated every day from the same location for an entire year. The performance of three types of samplers are evaluated assuming they are located at 15 IMS radionuclide stations in the region of the release point. The performance of two IMS-deployed samplers and a next-generation system is compared with proposed metrics for detection and discrimination using representative releases from the nuclear test site used by the Democratic People's Republic of Korea.
《全面禁止核试验条约》禁止所有核试验,并要求制定核查措施以探测违反条约的行为。一种核查措施是探测锕系元素裂变产生的放射性氙同位素。国际监测系统(IMS)目前部署了能够探测四种放射性氙同位素的自动放射性氙系统。目前正在开发具有更低探测限的放射性氙系统。从历史上看,放射性氙系统的灵敏度是通过每种同位素的最低可探测浓度来衡量的。在本文中,我们结合指示地下核爆炸的假设代表性释放,使用严格的指标来分析放射性氙系统的响应,而不是仅使用最低可探测浓度。我们的分析纳入了潜在光谱干扰对探测限的影响,以及测量相关放射性氙同位素的同位素比对于改善与背景源的区分的重要性,特别是对于低水平释放。为了提供足够的分析数据集,全年每天从同一地点模拟假设的代表性释放。假设三种类型的采样器位于释放点区域的15个IMS放射性核素站,对其性能进行评估。将两种IMS部署的采样器和一种下一代系统的性能与使用朝鲜核试验场的代表性释放进行探测和区分的拟议指标进行比较。