Shimojima Takahiro, Malaeb Walid, Nakamura Asuka, Kondo Takeshi, Kihou Kunihiro, Lee Chul-Ho, Iyo Akira, Eisaki Hiroshi, Ishida Shigeyuki, Nakajima Masamichi, Uchida Shin-Ichi, Ohgushi Kenya, Ishizaka Kyoko, Shin Shik
Quantum-Phase Electronics Center and Department of Applied Physics, University of Tokyo, Bunkyo, Tokyo 113-8656, Japan.
Institute for Solid State Physics, University of Tokyo, Kashiwa, Chiba 277-8581, Japan.
Sci Adv. 2017 Aug 25;3(8):e1700466. doi: 10.1126/sciadv.1700466. eCollection 2017 Aug.
A major problem in the field of high-transition temperature () superconductivity is the identification of the electronic instabilities near superconductivity. It is known that the iron-based superconductors exhibit antiferromagnetic order, which competes with the superconductivity. However, in the nonmagnetic state, there are many aspects of the electronic instabilities that remain unclarified, as represented by the orbital instability and several in-plane anisotropic physical properties. We report a new aspect of the electronic state of the optimally doped iron-based superconductors by using high-energy resolution angle-resolved photoemission spectroscopy. We find spectral evidence for the folded electronic structure suggestive of an antiferroic electronic instability, coexisting with the superconductivity in the nonmagnetic state of Ba K FeAs. We further establish a phase diagram showing that the antiferroic electronic structure persists in a large portion of the nonmagnetic phase covering the superconducting dome. These results motivate consideration of a key unknown electronic instability, which is necessary for the achievement of high- superconductivity in the iron-based superconductors.
高温超导领域的一个主要问题是确定超导附近的电子不稳定性。已知铁基超导体表现出反铁磁序,它与超导相互竞争。然而,在非磁性状态下,电子不稳定性的许多方面仍未得到阐明,如轨道不稳定性和一些面内各向异性物理性质所体现的那样。我们通过使用高能量分辨率角分辨光电子能谱,报告了最佳掺杂铁基超导体电子态的一个新方面。我们发现了折叠电子结构的光谱证据,这暗示着反铁电电子不稳定性,在BaKFeAs的非磁性状态下与超导共存。我们进一步建立了一个相图,表明反铁电电子结构在覆盖超导穹顶的大部分非磁性相中持续存在。这些结果促使人们考虑一个关键的未知电子不稳定性,这对于在铁基超导体中实现高温超导是必要的。