Samarakoon A M, Takahashi M, Zhang D, Yang J, Katayama N, Sinclair R, Zhou H D, Diallo S O, Ehlers G, Tennant D A, Wakimoto S, Yamada K, Chern G-W, Sato T J, Lee S-H
Department of Physics, University of Virginia, Charlottesville, Virginia, 22904, USA.
Oak Ridge National Laboratory, Oak Ridge, Tennessee, 37831, USA.
Sci Rep. 2017 Sep 21;7(1):12053. doi: 10.1038/s41598-017-12187-9.
Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of [Formula: see text]. This exponent is different from [Formula: see text] of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from [Formula: see text] of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid.
在自然界中,玻璃态无处不在且具有多样的特性。了解它们的差异和分类仍然是一项重大的科学挑战。在此,我们表明,磁记忆随时间的标度可用于将磁性玻璃态材料分为两个不同的类别。所研究的体系包括高温超导相关材料、自旋轨道莫特绝缘体、受挫磁体和稀磁合金。我们的体磁化测量结果表明,大多数高密度磁体表现出相似的记忆行为,其特征在于弛豫指数为[公式:见原文]。该指数不同于稀磁合金的[公式:见原文],后者归因于它们的分层和分形能量景观,并且也不同于自旋固体(一种具有长程有序的状态)预期的传统德拜弛豫的[公式:见原文]。此外,我们对具有不同磁浓度的稀磁合金进行的系统研究显示了两种玻璃态和自旋固体之间的转变。